Three-Dimensional Macroscopic Assemblies of Low-Dimensional Carbon Nitrides for Enhanced Hydrogen Evolution

被引:407
作者
Jun, Young-Si [1 ]
Park, Jihee [1 ]
Lee, Sun Uk [3 ]
Thomas, Arne [2 ]
Hong, Won Hi [3 ]
Stucky, Galen D. [1 ]
机构
[1] Univ Calif Santa Barbara, Dept Chem & Biochem, Santa Barbara, CA 93106 USA
[2] Tech Univ Berlin, Dept Chem Funct Mat, D-10623 Berlin, Germany
[3] Korea Adv Inst Sci & Technol, Dept Chem & Biomol Engn, Taejon 305701, South Korea
关键词
carbon nitrides; crystal engineering; hydrogen-bonded networks; photocatalysis; supramolecular chemistry; GRAPHENE; NANOPARTICLES; NANOSHEETS; MOLECULES; NETWORKS;
D O I
10.1002/anie.201304034
中图分类号
O6 [化学];
学科分类号
070301 [无机化学];
摘要
Simple organic cooperative assembly of triazine molecules leads to three-dimensional macroscopic assemblies of low-dimensional graphitic carbon nitrides (g-CNs), for example, nanoparticles, nanotubes, and nanosheets. The approach enables the characterization of the cooperative properties and photocatalytic activities of low-dimensional g-CN materials in hydrogen evolution reactions from water under visible light. Copyright © 2013 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
引用
收藏
页码:11083 / 11087
页数:5
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