Hydrogen evolution across nano-Schottky junctions at carbon supported MoS2 catalysts in biphasic liquid systems

被引:109
作者
Ge, Peiyu [1 ]
Scanlon, Micheal D. [1 ]
Peljo, Pekka [2 ]
Bian, Xiaojun [3 ]
Vubrel, Heron [4 ]
O'Neill, Arlene [5 ,6 ]
Coleman, Jonathan N. [5 ,6 ]
Cantoni, Marco [7 ]
Hu, Xile [4 ]
Kontturi, Kyosti [2 ]
Liu, BaoHong [3 ]
Girault, Hubert H. [1 ]
机构
[1] Ecole Polytech Fed Lausanne, LEPA, CH-1015 Lausanne, Switzerland
[2] Aalto Univ, Dept Chem, Helsinki 00076, Finland
[3] Fudan Univ, Inst Biomed Sci, Dept Chem, Shanghai 200433, Peoples R China
[4] Ecole Polytech Fed Lausanne, LISC, CH-1015 Lausanne, Switzerland
[5] Univ Dublin Trinity Coll, Sch Phys, Dublin D2, Ireland
[6] Univ Dublin Trinity Coll, Ctr Res Adapt Nanostruct & Nanodevices, Dublin D2, Ireland
[7] Ecole Polytech Fed Lausanne, Interdisciplinary Ctr Elect Microscopy CIME, CH-1015 Lausanne, Switzerland
基金
欧洲研究理事会; 芬兰科学院;
关键词
REDUCTION; DECAMETHYLFERROCENE; OXYGEN;
D O I
10.1039/c2cc31398g
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
The activities of a series of MoS2-based hydrogen evolution catalysts were studied by biphasic reactions monitored by UV/Vis spectroscopy. Carbon supported MoS2 catalysts performed best due to an abundance of catalytic edge sites and strong electronic coupling of catalyst to support.
引用
收藏
页码:6484 / 6486
页数:3
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