Lane formation in colloidal mixtures driven by an external field -: art. no. 021402

被引:183
作者
Dzubiella, J [1 ]
Hoffmann, GP [1 ]
Löwen, H [1 ]
机构
[1] Univ Dusseldorf, Inst Theoret Phys 2, D-40225 Dusseldorf, Germany
关键词
D O I
10.1103/PhysRevE.65.021402
中图分类号
O35 [流体力学]; O53 [等离子体物理学];
学科分类号
070204 ; 080103 ; 080704 ;
摘要
The influence of an external field on a binary colloidal mixture performing Brownian dynamics in a solvent is investigated by nonequilibrium computer simulations and simple theory. In our model, one half of the particles are pushed into the field direction while the other half of them are pulled into the opposite direction. For increasing field strength, we show that the system undergoes a nonequilibrium phase transition from a disordered state to a state characterized by lane formation parallel to the field direction. The lanes are formed by the same kind of particles moving collectively with the field. Lane formation accelerates particle transport parallel to the field direction but suppresses massively transport perpendicular to the field. We further show that lane formation also occurs in a time-dependent oscillatory field. If the frequency of the external field exceeds a critical value, however, the system exhibits a transition back to the disordered state. Our results can be experimentally verified in binary colloidal suspensions exposed to external fields under nonequilibrium conditions.
引用
收藏
页码:1 / 021402
页数:8
相关论文
共 48 条
[21]   STRUCTURE AND BROWNIAN DYNAMICS OF THE 2-DIMENSIONAL YUKAWA FLUID [J].
LOWEN, H .
JOURNAL OF PHYSICS-CONDENSED MATTER, 1992, 4 (50) :10105-10116
[22]   BROWNIAN DYNAMICS AND KINETIC GLASS-TRANSITION IN COLLOIDAL SUSPENSIONS [J].
LOWEN, H ;
HANSEN, JP ;
ROUX, JN .
PHYSICAL REVIEW A, 1991, 44 (02) :1169-1181
[23]   DYNAMIC CRITERION FOR FREEZING OF COLLOIDAL LIQUIDS [J].
LOWEN, H ;
PALBERG, T ;
SIMON, R .
PHYSICAL REVIEW LETTERS, 1993, 70 (10) :1557-1560
[24]   Colloidal soft matter under external control [J].
Löwen, H .
JOURNAL OF PHYSICS-CONDENSED MATTER, 2001, 13 (24) :R415-R432
[25]   MELTING, FREEZING AND COLLOIDAL SUSPENSIONS [J].
LOWEN, H .
PHYSICS REPORTS-REVIEW SECTION OF PHYSICS LETTERS, 1994, 237 (05) :249-324
[26]   LONG-TIME SELF-DIFFUSION COEFFICIENT IN COLLOIDAL SUSPENSIONS - THEORY VERSUS SIMULATION [J].
LOWEN, H ;
SZAMEL, G .
JOURNAL OF PHYSICS-CONDENSED MATTER, 1993, 5 (15) :2295-2306
[27]   Possibilities of phase separation in colloidal suspensions [J].
Lowen, H .
PHYSICA A, 1997, 235 (1-2) :129-141
[28]   Melting of polydisperse colloidal crystals in nonequilibrium [J].
Löwen, H ;
Hoffmann, GP .
PHYSICAL REVIEW E, 1999, 60 (03) :3009-3014
[29]   Experimental observations of non-Gaussian behavior and stringlike cooperative dynamics in concentrated quasi-two-dimensional colloidal liquids [J].
Marcus, AH ;
Schofield, J ;
Rice, SA .
PHYSICAL REVIEW E, 1999, 60 (05) :5725-5736
[30]  
Marro J., 1999, NONEQUILIBRIUM PHASE