Scavenging of pollutant acid substances by Asian mineral dust particles

被引:22
作者
Matsumoto, J
Takahashi, K
Matsumi, Y
Yabushita, A
Shimizu, A
Matsui, I
Sugimoto, N
机构
[1] Natl Inst Environm Sci, Tsukuba, Ibaraki 3058506, Japan
[2] Horiba Ltd, Kyoto 6018510, Japan
关键词
D O I
10.1029/2006GL025782
中图分类号
P [天文学、地球科学];
学科分类号
07 ;
摘要
Uptakes of sulfate and nitrate onto Asian dust particles during transport from the Asian continent to the Pacific Ocean were analyzed by using a single-particle time-of-flight mass spectrometer. Observation was conducted at Tsukuba in Japan in the springtime of 2004. Sulfate-rich dust particles made their largest contribution during the 'dust event' in the middle of April 2004. As a result of detailed analysis including backward trajectory calculations, it was confirmed that sulfate components originating from coal combustion in the continent were internally mixed with dust particles. Even in the downstream of the outflow far from the continental coastline, significant contribution of Asian dust to sulfate was observed. Asian dust plays critical roles as the carrier of sulfate over the Pacific Ocean.
引用
收藏
页数:4
相关论文
共 22 条
[1]   DISTRIBUTION OF SO2, NOX AND CO2 EMISSIONS FROM FUEL COMBUSTION AND INDUSTRIAL ACTIVITIES IN ASIA WITH 1-DEGREES-X1-DEGREES RESOLUTION [J].
AKIMOTO, H ;
NARITA, H .
ATMOSPHERIC ENVIRONMENT, 1994, 28 (02) :213-225
[2]   Marine boundary layer dust and pollutant transport associated with the passage of a frontal system over eastern Asia [J].
Bates, TS ;
Quinn, PK ;
Coffman, DJ ;
Covert, DS ;
Miller, TL ;
Johnson, JE ;
Carmichael, GR ;
Uno, I ;
Guazzotti, SA ;
Sodeman, DA ;
Prather, KA ;
Rivera, M ;
Russell, LM ;
Merrill, JT .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2004, 109 (D19) :D19S191-18
[3]   Asian dust storm events of spring 2001 and associated pollutants observed in New England by the Atmospheric Investigation, Regional Modeling, Analysis and Prediction (AIRMAP) monitoring network [J].
DeBell, LJ ;
Vozzella, M ;
Talbot, RW ;
Dibb, JE .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2004, 109 (D1)
[4]   Health impacts of coal and coal use: possible solutions [J].
Finkelman, RB ;
Orem, W ;
Castranova, V ;
Tatu, CA ;
Belkin, HE ;
Zheng, BS ;
Lerch, HE ;
Maharaj, SV ;
Bates, AL .
INTERNATIONAL JOURNAL OF COAL GEOLOGY, 2002, 50 (1-4) :425-443
[5]   Real-time analysis of individual atmospheric aerosol particles: Design and performance of a portable ATOFMS [J].
Gard, E ;
Mayer, JE ;
Morrical, BD ;
Dienes, T ;
Fergenson, DP ;
Prather, KA .
ANALYTICAL CHEMISTRY, 1997, 69 (20) :4083-4091
[6]   An overview of ACE-Asia: Strategies for quantifying the relationships between Asian aerosols and their climatic impacts [J].
Huebert, BJ ;
Bates, T ;
Russell, PB ;
Shi, GY ;
Kim, YJ ;
Kawamura, K ;
Carmichael, G ;
Nakajima, T .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2003, 108 (D23)
[7]   Development of an aerosol mass spectrometer for size and composition analysis of submicron particles [J].
Jayne, JT ;
Leard, DC ;
Zhang, XF ;
Davidovits, P ;
Smith, KA ;
Kolb, CE ;
Worsnop, DR .
AEROSOL SCIENCE AND TECHNOLOGY, 2000, 33 (1-2) :49-70
[8]   A comparison of particle mass spectrometers during the 1999 Atlanta Supersite Project [J].
Middlebrook, AM ;
Murphy, DM ;
Lee, SH ;
Thomson, DS ;
Prather, KA ;
Wenzel, RJ ;
Liu, DY ;
Phares, DJ ;
Rhoads, KP ;
Wexler, AS ;
Johnston, MV ;
Jimenez, JL ;
Jayne, JT ;
Worsnop, DR ;
Yourshaw, I ;
Seinfeld, JH ;
Flagan, RC .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2003, 108 (D7)
[9]   Change in size distribution and chemical composition of kosa (Asian dust) aerosol during long-range transport [J].
Mori, I ;
Nishikawa, M ;
Tanimura, T ;
Quan, H .
ATMOSPHERIC ENVIRONMENT, 2003, 37 (30) :4253-4263
[10]   LASER IONIZATION MASS-SPECTROSCOPY OF SINGLE AEROSOL-PARTICLES [J].
MURPHY, DM ;
THOMSON, DS .
AEROSOL SCIENCE AND TECHNOLOGY, 1995, 22 (03) :237-249