25th Anniversary Article: Colloidal Quantum Dot Materials and Devices: A Quarter-Century of Advances

被引:413
作者
Kim, Jin Young [1 ]
Voznyy, Oleksandr [1 ]
Zhitomirsky, David [1 ]
Sargent, Edward H. [1 ]
机构
[1] Univ Toronto, Dept Elect & Comp Engn, Toronto, ON M5S 3G4, Canada
基金
加拿大自然科学与工程研究理事会;
关键词
colloidal quantum dots; optoelectronics; solar cells; light emission; photodetectors; MULTIPLE EXCITON GENERATION; CORE-SHELL NANOCRYSTALS; BAND-LIKE TRANSPORT; ONE-POT SYNTHESIS; SEMICONDUCTOR NANOCRYSTALS; CARRIER-MULTIPLICATION; SOLAR-CELLS; CDSE NANOCRYSTALS; CHARGE-TRANSPORT; FLUORESCENCE INTERMITTENCY;
D O I
10.1002/adma.201301947
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Colloidal quantum dot (CQD) optoelectronics offers a compelling combination of low-cost, large-area solution processing, and spectral tunability through the quantum size effect. Since early reports of size-tunable light emission from solution-synthesized CQDs over 25 years ago, tremendous progress has been made in synthesis and assembly, optical and electrical properties, materials processing, and optoelectronic applications of these materials. Here some of the major developments in this field are reviewed, touching on key milestones as well as future opportunities.
引用
收藏
页码:4986 / 5010
页数:25
相关论文
共 218 条
[1]   Highly photoluminescent PbS nanocrystals: The beneficial effect of trioctylphosphine [J].
Abel, Keith A. ;
Shan, Jingning ;
Boyer, John-Christopher ;
Harris, Fraser ;
van Veggel, Frank C. J. M. .
CHEMISTRY OF MATERIALS, 2008, 20 (12) :3794-3796
[2]   ELECTRONIC STATES OF SEMICONDUCTOR CLUSTERS - HOMOGENEOUS AND INHOMOGENEOUS BROADENING OF THE OPTICAL-SPECTRUM [J].
ALIVISATOS, AP ;
HARRIS, AL ;
LEVINOS, NJ ;
STEIGERWALD, ML ;
BRUS, LE .
JOURNAL OF CHEMICAL PHYSICS, 1988, 89 (07) :4001-4011
[3]   Confinement effects in PbSe quantum wells and nanocrystals [J].
Allan, G ;
Delerue, C .
PHYSICAL REVIEW B, 2004, 70 (24) :1-9
[4]   The excitonic exchange splitting and radiative lifetime in PbSe quantum dots [J].
An, J. M. ;
Franceschetti, A. ;
Zunger, A. .
NANO LETTERS, 2007, 7 (07) :2129-2135
[5]   Soluble, Chloride-Terminated CdSe Nanocrystals: Ligand Exchange Monitored by 1H and 31P NMR Spectroscopy [J].
Anderson, Nicholas C. ;
Owen, Jonathan S. .
CHEMISTRY OF MATERIALS, 2013, 25 (01) :69-76
[6]   Identification of atomic-like electronic states in indium arsenide nanocrystal quantum dots [J].
Banin, U ;
Cao, YW ;
Katz, D ;
Millo, O .
NATURE, 1999, 400 (6744) :542-544
[7]   Electronic states and optical properties of PbSe nanorods and nanowires [J].
Bartnik, A. C. ;
Efros, Al. L. ;
Koh, W. -K. ;
Murray, C. B. ;
Wise, F. W. .
PHYSICAL REVIEW B, 2010, 82 (19)
[8]   Formation of high quality InP and InAs nanocrystals in a noncoordinating solvent [J].
Battaglia, D ;
Peng, XG .
NANO LETTERS, 2002, 2 (09) :1027-1030
[9]   THE QUANTUM-MECHANICS OF LARGER SEMICONDUCTOR CLUSTERS (QUANTUM DOTS) [J].
BAWENDI, MG ;
STEIGERWALD, ML ;
BRUS, LE .
ANNUAL REVIEW OF PHYSICAL CHEMISTRY, 1990, 41 :477-496
[10]   Multiple exciton generation in semiconductor nanocrystals: Toward efficient solar energy conversion [J].
Beard, Matthew C. ;
Ellingson, Randy J. .
LASER & PHOTONICS REVIEWS, 2008, 2 (05) :377-399