Critical review and meta-analysis of ambient particulate matter source apportionment using receptor models in Europe

被引：474

作者：

Belis, C. A. ^{[1
]}

Karagulian, F. ^{[1
]}

Larsen, B. R. ^{[2
]}

Hopke, P. K. ^{[3
]}

机构：

[1] Commiss European Communities, Joint Res Ctr, Inst Environm & Sustainabil, I-21027 Ispra, VA, Italy

[2] Commiss European Communities, Joint Res Ctr, Inst Hlth & Consumer Protect, I-21027 Ispra, VA, Italy

[3] Clarkson Univ, Ctr Air Resources Engn & Sci, Potsdam, NY 13699 USA

来源：

ATMOSPHERIC ENVIRONMENT | 2013年 / 69卷

关键词：

PM10; PM2.5; Particulate matter; Source apportionment; Receptor models; Europe; Exceedances; Carbonaceous fraction; Particulate organic carbon; POSITIVE MATRIX FACTORIZATION; PM10 SOURCE APPORTIONMENT; CHEMICAL MASS-BALANCE; PRINCIPAL COMPONENT ANALYSIS; AIR-POLLUTION SOURCES; ORGANIC-AEROSOL; LEAST-SQUARES; URBAN AREA; SOURCE IDENTIFICATION; METAL CONCENTRATIONS;

D O I：

10.1016/j.atmosenv.2012.11.009

中图分类号：

X [环境科学、安全科学];

学科分类号：

08 ; 0830 ;

摘要：

A review was conducted of the published literature on source apportionment of ambient particulate matter (PM) in Europe using receptor models (RMs). Consistent records were identified for source contribution estimates of PM mass concentrations for 272 records and of organic carbon (OC) in PM for 60 records. Over the period 2000-2012, a shift was observed in the use of RMs from principal component analysis, enrichment factors, and classical factor analysis to Positive Matrix Factorization while Chemical Mass Balance is still topical. Following a meta-analysis of the published results, six major source categories for PM were defined that comprise almost all individual sources apportioned in Europe: atmospheric formation of secondary inorganic aerosol (SIA), traffic, re-suspension of crustal/mineral dust, biomass burning, (industrial) point sources, and sea/road salt. For the OC fraction, the three main source categories were: atmospheric formation of secondary organic aerosol, biomass burning, and fossil fuel combustion. The geographical and seasonal variations of these sources are mapped and discussed. A special analysis of PM concentrations that exceed the current European air quality limits indicated SIA and traffic as the most important source categories to target for abatement throughout the year together with biomass burning during the cold season. (C) 2012 Elsevier Ltd. All rights reserved.

引用

页码：94 / 108

页数：15

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