Probing single molecule kinetics by photon arrival trajectories

被引：25

作者：

Barsegov, V ^{[1
]}

Mukamel, S ^{[1
]}

机构：

[1] Univ Rochester, Dept Chem, Rochester, NY 14627 USA

来源：

JOURNAL OF CHEMICAL PHYSICS | 2002年 / 116卷 / 22期

关键词：

D O I：

10.1063/1.1475751

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

Multitime correlation functions of photon arrival times in single molecule fluorescence resonant energy transfer measurements are computed using a simple model representing slow conformational dynamics described by a collective stochastic Gaussian coordinate. The analogy with time domain nonlinear optical spectroscopy is explored. Various statistical measures of distributions of single photon arrival times and fluorescence lifetimes are employed to analyze non-Poissonian statistics. (C) 2002 American Institute of Physics.

引用

页码：9802 / 9810

页数：9

共 41 条

[1] [Anonymous], RANDOM WALKS RANDOM
[2] Time-dependent fluctuations in single molecule spectroscopy: A generalized Wiener-Khintchine approach
Barkai, E
Jung, Y
Silbey, R
[J]. PHYSICAL REVIEW LETTERS, 2001, 87 (20) : 207403 - 1
[3] Multitime correlation functions for single molecule kinetics with fluctuating bottlenecks
Barsegov, V
Chernyak, V
Mukamel, S
[J]. JOURNAL OF CHEMICAL PHYSICS, 2002, 116 (10) : 4240 - 4251
[4] ANOMALOUS DIFFUSION IN DISORDERED MEDIA - STATISTICAL MECHANISMS, MODELS AND PHYSICAL APPLICATIONS
BOUCHAUD, JP
GEORGES, A
[J]. PHYSICS REPORTS-REVIEW SECTION OF PHYSICS LETTERS, 1990, 195 (4-5): : 127 - 293
[5] Single-molecule identification of Coumarin-120 by time-resolved fluorescence detection: Comparison of one- and two-photon excitation in solution
Brand, L
Eggeling, C
Zander, C
Drexhage, KH
Seidel, CAM
[J]. JOURNAL OF PHYSICAL CHEMISTRY A, 1997, 101 (24) : 4313 - 4321
[6] Rabi resonances of a single molecule driven by rf and laser fields
Brunel, C
Lounis, B
Tamarat, P
Orrit, M
[J]. PHYSICAL REVIEW LETTERS, 1998, 81 (13) : 2679 - 2682
[7] Stochastic-trajectories and nonPoisson kinetics in single-molecule spectroscopy
Chernyak, V
Schulz, M
Mukamel, S
[J]. JOURNAL OF CHEMICAL PHYSICS, 1999, 111 (16) : 7416 - 7425
[8] Three-dimensional imaging of single molecules solvated in pores of poly(acrylamide) gels
Dickson, RM
Norris, DJ
Tzeng, YL
Moerner, WE
[J]. SCIENCE, 1996, 274 (5289) : 966 - 969
[9] NONCLASSICAL RADIATION OF A SINGLE STORED ION
DIEDRICH, F
WALTHER, H
[J]. PHYSICAL REVIEW LETTERS, 1987, 58 (03) : 203 - 206
[10] Conformational transitions monitored for single molecules in solution
Edman, L
Mets, U
Rigler, R
[J]. PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 1996, 93 (13) : 6710 - 6715

← 1 2 3 4 5 →