Probing single molecule kinetics by photon arrival trajectories

被引：25

作者：

Barsegov, V ^{[1
]}

Mukamel, S ^{[1
]}

机构：

[1] Univ Rochester, Dept Chem, Rochester, NY 14627 USA

来源：

JOURNAL OF CHEMICAL PHYSICS | 2002年 / 116卷 / 22期

关键词：

D O I：

10.1063/1.1475751

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

Multitime correlation functions of photon arrival times in single molecule fluorescence resonant energy transfer measurements are computed using a simple model representing slow conformational dynamics described by a collective stochastic Gaussian coordinate. The analogy with time domain nonlinear optical spectroscopy is explored. Various statistical measures of distributions of single photon arrival times and fluorescence lifetimes are employed to analyze non-Poissonian statistics. (C) 2002 American Institute of Physics.

引用

页码：9802 / 9810

页数：9

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