Pore chemistry and size control in hybrid porous materials for acetylene capture from ethylene

被引:1012
作者
Cui, Xili [1 ]
Chen, Kaijie [2 ]
Xing, Huabin [1 ]
Yang, Qiwei [1 ]
Krishna, Rajamani [3 ]
Bao, Zongbi [1 ]
Wu, Hui [4 ]
Zhou, Wei [4 ]
Dong, Xinglong [5 ]
Han, Yu [5 ]
Li, Bin [6 ]
Ren, Qilong [1 ]
Zaworotko, Michael J. [2 ]
Chen, Banglin [6 ]
机构
[1] Zhejiang Univ, Coll Chem & Biol Engn, Minist Educ, Key Lab Biomass Chem Engn, Hangzhou 310027, Zhejiang, Peoples R China
[2] Univ Limerick, Dept Chem & Environm Sci, Limerick, Ireland
[3] Univ Amsterdam, Vant Hoff Inst Mol Sci, Sci Pk 904, NL-1098 XH Amsterdam, Netherlands
[4] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA
[5] King Abdullah Univ Sci & Technol, Phys Sci & Engn Div, Adv Membranes & Porous Mat Ctr, Thuwal 239556900, Saudi Arabia
[6] Univ Texas San Antonio, Dept Chem, One UTSA Circle, San Antonio, TX 78249 USA
基金
中国国家自然科学基金; 爱尔兰科学基金会;
关键词
METAL-ORGANIC FRAMEWORKS; METHANE STORAGE; CARBON-DIOXIDE; CO2; ADSORPTION; FUNCTIONALITIES; SEPARATION; REMOVAL;
D O I
10.1126/science.aaf2458
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
The trade-off between physical adsorption capacity and selectivity of porous materials is a major barrier for efficient gas separation and purification through physisorption. We report control over pore chemistry and size in metal coordination networks with hexafluorosilicate and organic linkers for the purpose of preferential binding and orderly assembly of acetylene molecules through cooperative host-guest and/or guest-guest interactions. The specific binding sites for acetylene are validated by modeling and neutron powder diffraction studies. The energies associated with these binding interactions afford high adsorption capacity (2.1 millimoles per gram at 0.025 bar) and selectivity (39.7 to 44.8) for acetylene at ambient conditions. Their efficiency for the separation of acetylene/ethylene mixtures is demonstrated by experimental breakthrough curves (0.73 millimoles per gram from a 1/99 mixture).
引用
收藏
页码:141 / 144
页数:4
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