Electric field tuning of plasmonic response of nanodot array in liquid crystal matrix

被引:237
作者
Kossyrev, PA
Yin, AJ
Cloutier, SG
Cardimona, DA
Huang, DH
Alsing, PM
Xu, JM
机构
[1] Brown Univ, Div Engn, Providence, RI 02912 USA
[2] Brown Univ, Dept Phys, Providence, RI 02912 USA
[3] USAF, Res Lab, Space Vehicles Directorate, Kirtland AFB, NM 87117 USA
关键词
D O I
10.1021/nl0513535
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
In this work we demonstrate the feasibility of electric-field tuning of the plasmonic spectrum of a novel gold nanodot array in a liquid crystal matrix. As opposed to previously reported microscopically observed near-field spectral tuning of individual gold nanoparticles, this system exhibits macroscopic far-field spectral tuning. The nanodot-liquid crystal matrix also displays strong anisotropic absorption characteristics, which can be effectively described as a collective ensemble within a composite matrix in the lateral dimension and a group of noninteracting individual particles in the normal direction. The effective medium model and the Mie theory are employed to describe the experimental results.
引用
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页码:1978 / 1981
页数:4
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