Real-world traffic emission factors of gases and particles measured in a road tunnel in Stockholm, Sweden

被引:221
作者
Kristensson, A
Johansson, C
Westerholm, R
Swietlicki, E
Gidhagen, L
Wideqvist, U
Vesely, V
机构
[1] Lund Univ, Div Nucl Phys, SE-22100 Lund, Sweden
[2] Stockholm Univ, Dept Analyt Chem, SE-10691 Stockholm, Sweden
[3] Swedish Meteorol & Hydrol Inst, SE-60176 Norrkoping, Sweden
[4] Stockholm Environm & Protect Agcy, SE-10064 Stockholm, Sweden
[5] Inst Appl Environm Res, ITM, Air Pollut Lab, SE-10691 Stockholm, Sweden
关键词
PM2.5; polycyclic aromatic hydrocarbons; particle size distribution; NOX; aldehydes;
D O I
10.1016/j.atmosenv.2003.10.030
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Measurements in a road tunnel in Stockholm, Sweden give the real-world traffic emission factors for a number of gaseous and particle pollutants. These include 49 different polycyclic aromatic hydrocarbons (PAH), CO, NOX, benzene, toluene, xylenes, aldehydes, elements and inorganic/organic carbon contained in particles, the sub-micrometer aerosol number size distribution, PM2.5 and PM10. The exhaust pipe emission factors are divided with the help of automated traffic counts into the two pollutant sources, the heavy-duty vehicles (HDV) and light-duty vehicles (LDV). The LDV fleet contains 95% petrol cars and the total fleet contains about 5% HDV. When data permitted, the emission factors were further calculated at different vehicle speeds. The current work shows that average CO, NOX and benzene emission factors amounted to 5.3, 1.4 and 0.017 g veh(-1) km(-1), respectively. Since the mid-90s CO and benzene decreased by about 15%, carbonyls by about a factor 2, whereas NOX did not change much. PAR emission factors were 2-15 times higher than found during dynamometer tests. Most particles are distributed around 20 nm diameter and the LDV fleet contributes to about 65% of both PM and particle number. In general, the gaseous emissions are higher in Sweden than in USA and Switzerland, foremost due to the lower fraction catalytic converters in Sweden. The PM and number emissions of particles are also slightly higher in the Swedish tunnel. (C) 2003 Elsevier Ltd. All rights reserved.
引用
收藏
页码:657 / 673
页数:17
相关论文
共 46 条
[21]  
Kirchstetter TW, 1999, ATMOS ENVIRON, V33, P2955
[22]   Impact of oxygenated gasoline use on California light-duty vehicle emissions [J].
Kirchstetter, TW ;
Singer, BC ;
Harley, RA ;
Kendall, GB ;
Chan, W .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 1996, 30 (02) :661-670
[23]  
KITTELSON D, 2000, SAE TECHNICAP PAPAER
[24]   Engines and nanoparticles: A review [J].
Kittelson, DB .
JOURNAL OF AEROSOL SCIENCE, 1998, 29 (5-6) :575-588
[25]  
KITTELSON DB, 2001, FINE PARTICLE EMISSI
[26]  
PALMGREN F, 1998, 6 INT S HIGHW URB PO
[27]   CONTINUOUS PM-10 MEASUREMENTS USING THE TAPERED ELEMENT OSCILLATING MICROBALANCE [J].
PATASHNICK, H ;
RUPPRECHT, EG .
JOURNAL OF THE AIR & WASTE MANAGEMENT ASSOCIATION, 1991, 41 (08) :1079-1083
[28]  
RUPPRECHT EG, 1995, AUTOMATED MONITOR ME
[29]   Real-world emissions and calculated reactivities of organic species from motor vehicles [J].
Sagebiel, JC ;
Zielinska, B ;
Pierson, WR ;
Gertler, AW .
ATMOSPHERIC ENVIRONMENT, 1996, 30 (12) :2287-2296
[30]   Measurement of emissions from air pollution sources.: 2.: C1 through C30 organic compounds from medium duty diesel trucks [J].
Schauer, JJ ;
Kleeman, MJ ;
Cass, GR ;
Simoneit, BRT .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 1999, 33 (10) :1578-1587