Conductivity fluctuation within a crystalline domain and its origin in pentacene thin-film transistors

被引:34
作者
Ohashi, Noboru [1 ]
Tomii, Hiroshi [1 ]
Matsubara, Ryousuke [1 ]
Sakai, Masatoshi [1 ]
Kudo, Kazuhiro [1 ]
Nakamura, Masakazu [1 ]
机构
[1] Chiba Univ, Grad Sch Engn, Dept Elect & Elect Engn, Chiba 2638522, Japan
关键词
D O I
10.1063/1.2799743
中图分类号
O59 [应用物理学];
学科分类号
摘要
Surface topography and high-resolution potential images in a thin-film transistor with a polycrystalline pentacene active layer have been measured by atomic-force-microscope potentiometry. A potential fluctuation independent of topographic features was found in large flat molecular terraces. The origin of the potential fluctuation was concluded to be the fluctuation of the top level of the highest-occupied-molecular-orbital band, which results in the variation of local carrier concentration. The full width at half maximum of the band fluctuation was estimated to be 12 meV, which might reduce the mean carrier velocity in crystalline domains. (C) 2007 American Institute of Physics.
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页数:3
相关论文
共 11 条
[1]   Grain size dependent mobility in polycrystalline organic field-effect transistors [J].
Horowitz, G ;
Hajlaoui, ME .
SYNTHETIC METALS, 2001, 122 (01) :185-189
[2]   Electronic structures of the highest occupied molecular orbital bands of a pentacene ultrathin film [J].
Kakuta, Haruya ;
Hirahara, Toru ;
Matsuda, Iwao ;
Nagao, Tadaaki ;
Hasegawa, Shuji ;
Ueno, Nobuo ;
Sakamoto, Kazuyuki .
PHYSICAL REVIEW LETTERS, 2007, 98 (24)
[3]   ELECTRONIC TRANSPORT IN AMORPHOUS SILICON FILMS [J].
LECOMBER, PG ;
SPEAR, WE .
PHYSICAL REVIEW LETTERS, 1970, 25 (08) :509-&
[4]  
MATSUBARA R, 2007, EXT ABSTR INT C SOL, P636
[5]   Atomic-scale sources and mechanism of nanoscale electronic disorder in Bi2Sr2CaCu2O8+δ [J].
McElroy, K ;
Lee, J ;
Slezak, JA ;
Lee, DH ;
Eisaki, H ;
Uchida, S ;
Davis, JC .
SCIENCE, 2005, 309 (5737) :1048-1052
[6]   Laser-based photoemission micro-spectroscopy for occupied and unoccupied states of inhomogeneous surfaces [J].
Munakata, T ;
Sugiyama, T ;
Sonoda, Y .
SURFACE SCIENCE, 2005, 593 (1-3) :38-42
[7]   Potential mapping of pentacene thin-film transistors using purely electric atomic-force-microscope potentiometry [J].
Nakamura, M ;
Goto, N ;
Ohashi, N ;
Sakai, M ;
Kudo, K .
APPLIED PHYSICS LETTERS, 2005, 86 (12) :1-3
[8]  
Nakamura M., 2005, IPAP C SERIES, V6, P130
[9]   Surface potential profiling and contact resistance measurements on operating pentacene thin-film transistors by Kelvin probe force microscopy [J].
Puntambekar, KP ;
Pesavento, PV ;
Frisbie, CD .
APPLIED PHYSICS LETTERS, 2003, 83 (26) :5539-5541
[10]  
STAUFFER D, 1994, INTRO PERCOLATION TH, P91