Characteristics of Black Carbon aerosols over Patiala Northwestern part of the IGP: Source apportionment using cluster and CWT analysis

被引:39
作者
Bonsal, Onam [1 ]
Singh, Atinderpal [1 ]
Singh, Darshan [1 ]
机构
[1] Punjabi Univ, Dept Phys, Patiala 147002, Punjab, India
关键词
Atmospheric boundary layer (ABL); Black Carbon (BC); Concentration Weighted Trajectory (CWT); Biomass burning; Indo-Gangetic Plain (IGP); LIGHT-ABSORPTION; THERMAL MEASUREMENTS; SPECTRAL DEPENDENCE; ELEMENTAL CARBON; ORGANIC-CARBON; URBAN LOCATION; BROWN CARBON; AMBIENT; PARTICLES; INDIA;
D O I
10.1016/j.apr.2018.08.001
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The present study represents the variation in characteristics of Black Carbon aerosols over Patiala (Punjab), northwest region of the IGP, India during two separate periods i.e. October 2013-September 2014 and October 2015-September 2016. Averaged BC mass concentration were found to be 9.9 mu g m(-3), 6.6 mu g m(-3), 3.4 mu g m(-3) and 2.8 mu g m(-3) during Autumn (Oct-Nov), Winter(Dec-March), Summer(Apr-June) and Monsoon (July-Aug) seasons respectively. During the entire study period, spectral dependence of aerosol mass absorption coefficient reveals that dominant source of BC is biomass burning during autumn season while there is mixed contribution from biomass, bio-fuel burning and fossil fuel combustion in rest of the seasons. These results are further supported by seasonal variations in Angstrom coefficient and Delta-C values. Averaged values of mass absorption efficiency of BC were found to be 3.8 m(2)g(-1), 5.0 m(2)g(-1), 5.6 m(2)g(-1) and 7.1 m(2)g(-1) during autumn, winter, summer and monsoon seasons respectively. Cluster & Concentration weighted trajectory (CWT) analysis suggests that potential sources of BC aerosol over the study region are local as well as transported from distant places mostly situated in the northwest, south-west and south-east side of the observation site depending upon the meteorological conditions and regional anthropogenic activities that varies with season. BC concentration derived from online MERRA-2 model for Patiala region and from global inventory EDGARHTAP site for agriculture waste burning further supports our findings.
引用
收藏
页码:244 / 256
页数:13
相关论文
共 53 条
[1]   The impact of natural versus anthropogenic aerosols on atmospheric circulation in the Community Atmosphere Model [J].
Allen, Robert J. ;
Sherwood, Steven C. .
CLIMATE DYNAMICS, 2011, 36 (9-10) :1959-1978
[2]   Black carbon or brown carbon?: The nature of light-absorbing carbonaceous aerosols [J].
Andreae, M. O. ;
Gelencser, A. .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2006, 6 :3131-3148
[3]   Variation in aerosol black carbon concentration and its emission estimates at the mega-city Delhi [J].
Bano, Tarannum ;
Singh, Sachchidanand ;
Gupta, N. C. ;
Soni, Kirti ;
Tanwar, R. S. ;
Nath, S. ;
Arya, B. C. ;
Gera, B. S. .
INTERNATIONAL JOURNAL OF REMOTE SENSING, 2011, 32 (21) :6749-6764
[4]   Influence of aerosol dry deposition on photosynthetically active radiation available to plants: A case study in the Yangtze delta region of China [J].
Bergin, MH ;
Greenwald, R ;
Xu, J ;
Berta, Y ;
Chameides, WL .
GEOPHYSICAL RESEARCH LETTERS, 2001, 28 (18) :3605-3608
[5]  
Bergstrom R. W., 1982, OPTICAL PROPERTIES P
[6]   Bounding the role of black carbon in the climate system: A scientific assessment [J].
Bond, T. C. ;
Doherty, S. J. ;
Fahey, D. W. ;
Forster, P. M. ;
Berntsen, T. ;
DeAngelo, B. J. ;
Flanner, M. G. ;
Ghan, S. ;
Kaercher, B. ;
Koch, D. ;
Kinne, S. ;
Kondo, Y. ;
Quinn, P. K. ;
Sarofim, M. C. ;
Schultz, M. G. ;
Schulz, M. ;
Venkataraman, C. ;
Zhang, H. ;
Zhang, S. ;
Bellouin, N. ;
Guttikunda, S. K. ;
Hopke, P. K. ;
Jacobson, M. Z. ;
Kaiser, J. W. ;
Klimont, Z. ;
Lohmann, U. ;
Schwarz, J. P. ;
Shindell, D. ;
Storelvmo, T. ;
Warren, S. G. ;
Zender, C. S. .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2013, 118 (11) :5380-5552
[7]   Light absorption by carbonaceous particles: An investigative review [J].
Bond, TC ;
Bergstrom, RW .
AEROSOL SCIENCE AND TECHNOLOGY, 2006, 40 (01) :27-67
[8]   Spectral dependence of visible light absorption by carbonaceous particles emitted from coal combustion [J].
Bond, TC .
GEOPHYSICAL RESEARCH LETTERS, 2001, 28 (21) :4075-4078
[9]   Changes to the Chemical Composition of Soot from Heterogeneous Oxidation Reactions [J].
Browne, Eleanor C. ;
Franklin, Jonathan P. ;
Canagaratna, Manjula R. ;
Massoli, Paola ;
Kirchstetter, Thomas W. ;
Worsnop, Douglas R. ;
Wilson, Kevin R. ;
Kroll, Jesse H. .
JOURNAL OF PHYSICAL CHEMISTRY A, 2015, 119 (07) :1154-1163
[10]   Case study of the effects of atmospheric aerosols and regional haze on agriculture: An opportunity to enhance crop yields in China through emission controls? [J].
Chameides, WL ;
Yu, H ;
Liu, SC ;
Bergin, M ;
Zhou, X ;
Mearns, L ;
Wang, G ;
Kiang, CS ;
Saylor, RD ;
Luo, C ;
Huang, Y ;
Steiner, A ;
Giorgi, F .
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 1999, 96 (24) :13626-13633