High-Mobility Conjugated Polymers Based on Fused-Thiophene Building Blocks

被引：94

作者：

Liu, Yao ^{[1
,2
,3
]}

Liu, Yunqi ^{[1
,2
]}

Zhan, Xiaowei ^{[1
,2
]}

机构：

[1] Chinese Acad Sci, Inst Chem, Beijing Natl Lab Mol Sci, Beijing 100190, Peoples R China

[2] Chinese Acad Sci, Inst Chem, Key Lab Organ Solids, Beijing 100190, Peoples R China

[3] Chinese Acad Sci, Grad Univ, Beijing 100049, Peoples R China

来源：

MACROMOLECULAR CHEMISTRY AND PHYSICS | 2011年 / 212卷 / 05期

关键词：

conjugated polymers; field-effect transistors; fused-thiophenes; mobilities; structure-property relations; FIELD-EFFECT TRANSISTORS; LOW-BAND-GAP; THIN-FILM TRANSISTORS; STACKED ORGANIC SEMICONDUCTOR; HIGH-PERFORMANCE; PHOTOVOLTAIC PROPERTIES; SOLAR-CELLS; LOW-TEMPERATURE; RAMAN-SPECTRA; BRIGHT FUTURE;

D O I：

10.1002/macp.201000677

中图分类号：

O63 [高分子化学（高聚物）];

学科分类号：

070305 ; 080501 ; 081704 ;

摘要：

Organic field-effect transistors (OFETs) are a promising cost-effective alternative to silicon-based field-effect transistors, and possess low-cost, light-weight, and flexibility advantages. Conjugated polymers based on fused-thiophene building blocks have received considerable attention in the emerging field of organic electronics. In this review the most recent developments in conjugated polymers based on fused-thiophene rings for high-performance OFETs are summarized. The focus is on correlations of polymer chemical structures with properties, such as energy levels, film-forming property, film morphology, and OFET performance. This structure-property relationship analysis may guide rational structural design and evaluation of organic semiconductors.

引用

页码：428 / 443

页数：16

共 139 条

[1] Organic semiconductors for solution-processable field-effect transistors (OFETs) [J].

Allard, Sybille ;

Forster, Michael ;

Souharce, Benjamin ;

Thiem, Heiko ;

Scherf, Ullrich .

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2008, 47 (22) :4070-4098

[2] Functionalized acenes and heteroacenes for organic electronics [J].

Anthony, John E. .

CHEMICAL REVIEWS, 2006, 106 (12) :5028-5048

[3] n-Type Organic Semiconductors in Organic Electronics [J].

Anthony, John E. ;

Facchetti, Antonio ;

Heeney, Martin ;

Marder, Seth R. ;

Zhan, Xiaowei .

ADVANCED MATERIALS, 2010, 22 (34) :3876-3892

[4] Materials and Applications for Large Area Electronics: Solution-Based Approaches [J].

Arias, Ana Claudia ;

MacKenzie, J. Devin ;

McCulloch, Iain ;

Rivnay, Jonathan ;

Salleo, Alberto .

CHEMICAL REVIEWS, 2010, 110 (01) :3-24

[5] Thienopyrazine-based low-bandgap poly(heteroaryleneethynylene)s for photovoltaic devices [J].

Ashraf, Raja Shahid ;

Shahid, Munazza ;

Klemm, Elisabeth ;

Al-Ibrahim, Maher ;

Sensfuss, Steffi .

MACROMOLECULAR RAPID COMMUNICATIONS, 2006, 27 (17) :1454-1459

[6]

Bao Z., 2006, Organic Field-Effect Transistors

[7] Tailoring Structure-Property Relationships in Dithienosilole-Benzothiadiazole Donor-Acceptor Copolymers [J].

Beaujuge, Pierre M. ;

Pisula, Wojciech ;

Tsao, Hoi Nok ;

Ellinger, Stefan ;

Muellen, Klaus ;

Reynolds, John R. .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2009, 131 (22) :7514-+

[8] Transistor and solar cell performance of donor-acceptor low bandgap copolymers bearing an acenaphtho[1,2-b]thieno[3,4-e]pyrazine (ACTP) motif [J].

Becerril, Hector A. ;

Miyaki, Nobuyuki ;

Tang, Ming Lee ;

Mondal, Rajib ;

Sun, Ya-Sen ;

Mayer, Alex C. ;

Parmer, Jack E. ;

McGehee, Michael D. ;

Bao, Zhenan .

JOURNAL OF MATERIALS CHEMISTRY, 2009, 19 (05) :591-593

[9] X-ray scattering study of thin films of poly(2,5-bis(3-alkylthiophen-2-yl)thieno[3,2-b]thiophene) [J].

Chabinyc, Michael L. ;

Toney, Michael F. ;

Kline, R. Joseph ;

McCulloch, Iain ;

Heeney, Martin .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2007, 129 (11) :3226-3237

[10] Poly(2,7-dibenzosilole): A blue light emitting polymer [J].

Chan, KL ;

McKiernan, MJ ;

Towns, CR ;

Holmes, AB .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2005, 127 (21) :7662-7663

← 1 2 3 4 5 6 7 8 9 10 →