Acrylic Acid Polymer Coatings on Silk Fibers by Room-temperature APGD Plasma Jets

被引:46
作者
Chen, Guangliang [1 ,2 ]
Zhou, Mingyan [3 ]
Zhang, Zhaoxia [1 ,2 ]
Lv, Guohua [4 ]
Massey, Sylvain [5 ]
Smith, Wilson [5 ]
Tatoulian, Michael [5 ]
机构
[1] Zhejiang Sci Tech Univ, Key Lab Adv Text Mat & Mfg Technol, Minist Educ, Hangzhou 310018, Peoples R China
[2] Zhejiang Sci Tech Univ, Engn Res Ctr Ecodyeing & Finishing Text, Minist Educ, Hangzhou 310018, Peoples R China
[3] Rensselaer Polytech Inst, Dept Civil & Environm Engn, Troy, NY 12180 USA
[4] Chinese Acad Sci, Inst Phys, Key Lab Soft Matter Phys, Beijing 100080, Peoples R China
[5] Univ Paris 06, Ecole Natl Super Chim Paris Chim ParisTech, Lab Genie Procedes Plasmas & Traitements Surfaces, F-75005 Paris, France
关键词
antimicrobial activity; APGD plasma jets; polymerization; silk fibers; ATMOSPHERIC-PRESSURE; SURFACE MODIFICATION; GLOW-DISCHARGE; HYDROPHOBICITY; DEPOSITION; FABRICS; SILICON; PLUME;
D O I
10.1002/ppap.201100008
中图分类号
O59 [应用物理学];
学科分类号
070305 [高分子化学与物理];
摘要
The aim of this work is to coat silk fibers (SF) with polymer of acrylic acid (PAA) using an atmospheric pressure glow discharge (APGD) plasma jet in order to immobilize antimicrobial peptide LL-37. The polymer properties are characterized by contact angle goniometry (CAG), XPS, AFM and SEM. The CA of the SF film can be decreased to 340, and the surface roughness of PAA in the center of plasma jet is larger than in other areas. Compared with the original SF, the concentration of carboxyl group increases greatly when the SF are modified by Ar plasma jet polymerization of AA. The augmentation of functional groups is very useful to immobilize larger concentrations of microbial peptide LL-37 on the SF surface, and the satisfactory antimicrobial activity on inhibiting the Escherichia coli (E. coli) is thereby achieved.
引用
收藏
页码:701 / 708
页数:8
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