Fine particle emissions from on-road vehicles in the Zhujiang Tunnel, China

被引:188
作者
He, Ling-Yan [2 ]
Hu, Min [1 ]
Zhang, Yuan-Hang [1 ]
Huang, Xiao-Feng [2 ]
Yao, Ting-Ting [2 ]
机构
[1] Peking Univ, Coll Environm Sci & Engn, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100871, Peoples R China
[2] Peking Univ, Shenzhen Grad Sch, Lab Environm & Urban Sci, Shenzhen 518055, Peoples R China
关键词
D O I
10.1021/es7022658
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Little is known about the characteristics of particulate matter emissions from vehicles in China, although such information is critical in source apportionment modeling, emission inventories, and health effect studies. In this paper, we report a comprehensive characterization Of PM2.5 emissions in the Zhujiang Tunnel in the Pearl River Delta region of China. The chemical speciation included elemental carbon, organic carbon, inorganic ions, trace elements, and organic compounds. The emission factors of individual species and their relative distributions were obtained for a mixed fleet of heavy-duty vehicles (19.8%) and light-duty vehicles (80.2%). In addition, separate emission factors of PM2.(5) mass, elemental carbon, and organic matter for heavy-duty vehicles and light-duty vehicles also were derived. As compared to the results of other tunnel studies previously conducted, we found that the abundances and distributions of the trace elements in PM2.5 emissions were more varied. In contrast, the characteristics of the trace organic compounds in the PM2.5 emissions in our study were consistent with characteristics found in other tunnel studies and dynamometer tests. Our results suggested that vehicular PM2.5 emissions of organic compounds are less influenced by the geographic area and fleet composition and thereby are more suitable for use in aerosol source apportionment modeling implemented across extensive regions.
引用
收藏
页码:4461 / 4466
页数:6
相关论文
共 43 条
  • [21] CHARACTERIZATION OF HEAVY-DUTY DIESEL VEHICLE EMISSIONS
    LOWENTHAL, DH
    ZIELINSKA, B
    CHOW, JC
    WATSON, JG
    GAUTAM, M
    FERGUSON, DH
    NEUROTH, GR
    STEVENS, KD
    [J]. ATMOSPHERIC ENVIRONMENT, 1994, 28 (04) : 731 - 743
  • [22] Characterization of polycyclic aromatic hydrocarbons in motor vehicle fuels and exhaust emissions
    Marr, LC
    Kirchstetter, TW
    Harley, RA
    Miguel, AH
    Hering, SV
    Hammond, SK
    [J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY, 1999, 33 (18) : 3091 - 3099
  • [24] On-road emissions of particulate polycyclic aromatic hydrocarbons and black carbon from gasoline and diesel vehicles
    Miguel, AH
    Kirchstetter, TW
    Harley, RA
    Hering, SV
    [J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY, 1998, 32 (04) : 450 - 455
  • [25] THE EFFECTS OF VEHICLE ACTIVITY ON PARTICLE RESUSPENSION
    NICHOLSON, KW
    BRANSON, JR
    GIESS, P
    CANNELL, RJ
    [J]. JOURNAL OF AEROSOL SCIENCE, 1989, 20 (08) : 1425 - 1428
  • [26] NIOSH, 1999, NIOSH MANUAL ANAL ME
  • [27] Identification and emission rates of molecular tracers in coal smoke particulate matter
    Oros, DR
    Simoneit, BRT
    [J]. FUEL, 2000, 79 (05) : 515 - 536
  • [28] Pollutants and asthma: Role of air toxics
    Peden, DB
    [J]. ENVIRONMENTAL HEALTH PERSPECTIVES, 2002, 110 : 565 - 568
  • [29] Real-world automotive emissions - Summary of studies in the Fort McHenry and Tuscarora Mountain Tunnels
    Pierson, WR
    Gertler, AW
    Robinson, NF
    Sagebiel, JC
    Zielinska, B
    Bishop, GA
    Stedman, DH
    Zweidinger, RB
    Ray, WD
    [J]. ATMOSPHERIC ENVIRONMENT, 1996, 30 (12) : 2233 - 2256
  • [30] SOURCES OF FINE ORGANIC AEROSOL .3. ROAD DUST, TIRE DEBRIS, AND ORGANOMETALLIC BRAKE LINING DUST - ROADS AS SOURCES AND SINKS
    ROGGE, WF
    HILDEMANN, LM
    MAZUREK, MA
    CASS, GR
    SIMONEIT, BRT
    [J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY, 1993, 27 (09) : 1892 - 1904