Spin-liquid behavior in a kagome antiferromagnet:: Deuteronium jarosite

被引:36
作者
Fak, B. [1 ,2 ]
Coomer, F. C. [3 ]
Harrison, A. [3 ]
Visser, D. [2 ,4 ]
Zhitomirsky, M. E. [1 ]
机构
[1] CEA Grenoble, SPSMS, Dept Rech Fondamentale Mat Condensee, F-38054 Grenoble, France
[2] Rutherford Appleton Lab, ISIS Facil, Didcot OX11 0QX, Oxon, England
[3] Univ Edinburgh, Sch Chem & EaStChem, Edinburgh EH9 3JJ, Midlothian, Scotland
[4] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England
关键词
D O I
10.1209/0295-5075/81/17006
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
The spin dynamics of the frustrated quasi-two-dimensional spin-5/2 Heisenberg antiferromagnetic kagome compound deuteronium jarosite, (D3O) Fe-3(SO4)(2)(OD)(6), has been studied using inelastic neutron scattering. The dynamic magnetic susceptibility shows a clear spin-liquid behavior with strong dynamic short-range correlations with staggered chirality, as seen from the wave vector dependence at finite-energy transfers. The magnetic scattering at low temperatures is gapless and extends out to at least 20 meV. The dynamics shows a non-exponential relaxation behavior but no dynamical w/T scaling. The characteristic energy (inverse relaxation rate) increases linearly with temperature. Copyright (C) EPLA, 2008.
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页数:6
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