Carbon content of atmospheric aerosols in a residential area during the wood combustion season in Sweden

被引:42
作者
Krecl, Patricia [1 ]
Stroem, Johan [1 ]
Johansson, Christer [1 ]
机构
[1] Stockholm Univ, Atmospher Sci Unit, Dept Appl Environm Sci, S-10691 Stockholm, Sweden
关键词
aethalometer; particle soot absorption photometer; elemental carbon; organic carbon; PM10;
D O I
10.1016/j.atmosenv.2007.06.025
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Carbonaceous aerosol particles were observed in a residential area with wood combustion during wintertime in Northern Sweden. Filter samples were analyzed for elemental carbon (EC) and organic carbon (OC) content by using a thermo-optical transmittance method. The light-absorbing carbon (LAC) content was determined by employing a commercial Aethalometer and a custom-built particle soot absorption photometer. Filter samples were used to convert the optical signals to LAC mass concentrations. Additional total PM10 mass concentrations and meteorological parameters were measured. The mean and standard deviation mass concentrations were 4.4 +/- 3.6 mu g m(-3) for OC, and 1.4 +/- 1.2 mu g m(-3) for EC. On average, EC accounted for 10.7% of the total PM10 and the contribution of OC to the total PM10 was 35.4%. Aethalometer and custom-built PSAP measurements were highly correlated (R 2 = 0.92). The hourly mean value of LAC mass concentration was 1.76 mu g m(-3) (median 0.88 mu g m(-3)) for the winter 2005-2006. This study shows that the custom-built PSAP is a reliable alternative for the commercial Aethalometer with the advantage of being a low-cost instrument. (c) 2007 Elsevier Ltd. All rights reserved.
引用
收藏
页码:6974 / 6985
页数:12
相关论文
共 33 条
[11]   Impact of wood combustion on particle levels in a residential area in Denmark [J].
Glasius, M. ;
Ketzel, M. ;
Wahlin, P. ;
Jensen, B. ;
Monster, J. ;
Berkowicz, R. ;
Palmgren, F. .
ATMOSPHERIC ENVIRONMENT, 2006, 40 (37) :7115-7124
[12]   THE AETHALOMETER - AN INSTRUMENT FOR THE REAL-TIME MEASUREMENT OF OPTICAL-ABSORPTION BY AEROSOL-PARTICLES [J].
HANSEN, ADA ;
ROSEN, H ;
NOVAKOV, T .
SCIENCE OF THE TOTAL ENVIRONMENT, 1984, 36 (JUN) :191-196
[13]   Chemical and physical characterization of emissions from birch wood combustion in a wood stove [J].
Hedberg, E ;
Kristensson, A ;
Ohlsson, M ;
Johansson, C ;
Johansson, PÅ ;
Swietlicki, E ;
Vesely, V ;
Wideqvist, U ;
Westerholm, R .
ATMOSPHERIC ENVIRONMENT, 2002, 36 (30) :4823-4837
[14]   Is levoglucosan a suitable quantitative tracer for wood burning? Comparison with receptor modeling on trace elements in Lycksele, Sweden [J].
Hedberg, Emma ;
Johansson, Christer .
JOURNAL OF THE AIR & WASTE MANAGEMENT ASSOCIATION, 2006, 56 (12) :1669-1678
[15]  
HEINTZENBERG J, 1987, Tellus Series B Chemical and Physical Meteorology, V39, P374, DOI 10.1111/j.1600-0889.1987.tb00200.x
[16]   Comparison of black carbon (BC) aerosols in two urban areas - concentrations and size distributions [J].
Hitzenberger, R ;
Tohno, S .
ATMOSPHERIC ENVIRONMENT, 2001, 35 (12) :2153-2167
[17]   Lidar, nephelometer, and in situ aerosol experiments in southern Ontario [J].
Hoff, RM ;
GuiseBagley, L ;
Staebler, RM ;
Wiebe, HA ;
Brook, J ;
Georgi, B ;
Dusterdiek, T .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1996, 101 (D14) :19199-19209
[18]   Emission characteristics of modern and old-type residential boilers fired with wood logs and wood pellets [J].
Johansson, LS ;
Leckner, B ;
Gustavsson, L ;
Cooper, D ;
Tullin, C ;
Potter, A .
ATMOSPHERIC ENVIRONMENT, 2004, 38 (25) :4183-4195
[19]   Evidence that the spectral dependence of light absorption by aerosols is affected by organic carbon [J].
Kirchstetter, TW ;
Novakov, T ;
Hobbs, PV .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2004, 109 (D21) :D212081-12
[20]  
KRISTENSSON A, 2005, THESIS LUND U LUND S