Simultaneous Optimization of Charge-Carrier Balance and Luminous Efficacy in Highly Efficient White Polymer Light-Emitting Devices

被引:201
作者
Zou, Jianhua [1 ]
Wu, Hao [2 ,3 ,7 ]
Lam, Ching-Shan [2 ,3 ,7 ]
Wang, Chuandao [4 ]
Zhu, Jing [4 ]
Zhong, Chengmei [1 ]
Hu, Sujun [1 ]
Ho, Cheuk-Lam [2 ,3 ,7 ]
Zhou, Gui-Jiang [5 ,6 ]
Wu, Hongbin [1 ]
Choy, Wallace C. H. [4 ]
Peng, Junbiao [1 ]
Cao, Yong [1 ]
Wong, Wai-Yeung [2 ,3 ,7 ]
机构
[1] S China Univ Technol, Inst Polymer Optoelect Mat & Devices, State Key Lab Optoelect Funct Mat & Devices, Guangzhou 510640, Guangdong, Peoples R China
[2] Hong Kong Baptist Univ, Dept Chem, Hong Kong, Hong Kong, Peoples R China
[3] Hong Kong Baptist Univ, Ctr Adv Luminescence Mat, Hong Kong, Hong Kong, Peoples R China
[4] Univ Hong Kong, Dept Elect & Elect Engn, Hong Kong, Hong Kong, Peoples R China
[5] Xi An Jiao Tong Univ, Fac Sci, Key Lab Nonequilibrium Synth & Modulat Condensed, Minist Educ, Xian 710049, Peoples R China
[6] Xi An Jiao Tong Univ, Fac Sci, Dept Chem, Xian 710049, Peoples R China
[7] Univ Grants Comm, Areas Excellence Scheme, Inst Mol Funct Mat, Hong Kong, Hong Kong, Peoples R China
基金
中国国家自然科学基金;
关键词
DIODES; EMISSION; EXCITONS;
D O I
10.1002/adma.201101130
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
White polymer light-emitting devices with a peak forward-viewing power efficiency close to 40 lm W-1, corresponding to an external quantum efficiency of 28.8% and a luminous efficiency of 60 cd A(-1), are demonstrated. The devices are based on two newly synthesized yellow-emitting iridium complexes functionalized with the sterically hindered diarylfluorene chromophores and are fabricated by a simple solution-processing method.
引用
收藏
页码:2976 / +
页数:6
相关论文
共 32 条
[1]   Highly efficient phosphorescent emission from organic electroluminescent devices [J].
Baldo, MA ;
O'Brien, DF ;
You, Y ;
Shoustikov, A ;
Sibley, S ;
Thompson, ME ;
Forrest, SR .
NATURE, 1998, 395 (6698) :151-154
[2]   Quantifying the efficiency of electrodes for positive carrier injection into poly(9,9-dioctylfluorene) and representative copolymers [J].
Campbell, AJ ;
Bradley, DDC ;
Antoniadis, H .
JOURNAL OF APPLIED PHYSICS, 2001, 89 (06) :3343-3351
[3]   White organic light-emitting devices for solid-state lighting [J].
D'Andrade, BW ;
Forrest, SR .
ADVANCED MATERIALS, 2004, 16 (18) :1585-1595
[4]   Efficient organic electrophosphorescent white-light-emitting device with a triple doped emissive layer [J].
D'Andrade, BW ;
Holmes, RJ ;
Forrest, SR .
ADVANCED MATERIALS, 2004, 16 (07) :624-+
[5]   On the origin of the color shift in white-emitting OLEDs [J].
Gather, Malte C. ;
Alle, Ronald ;
Becker, Heinrich ;
Meerholz, Klaus .
ADVANCED MATERIALS, 2007, 19 (24) :4460-+
[6]   White Organic Light-Emitting Diodes [J].
Gather, Malte C. ;
Koehnen, Anne ;
Meerholz, Klaus .
ADVANCED MATERIALS, 2011, 23 (02) :233-248
[7]   High-efficiency and low-voltage p-i-n electrophosphorescent organic light-emitting diodes with double-emission layers [J].
He, GF ;
Pfeiffer, M ;
Leo, K ;
Hofmann, M ;
Birnstock, J ;
Pudzich, R ;
Salbeck, J .
APPLIED PHYSICS LETTERS, 2004, 85 (17) :3911-3913
[8]   Highly Efficient Polymer White-Light-Emitting Diodes Based on Lithium Salts Doped Electron Transporting Layer [J].
Huang, Fei ;
Shih, Ping-I ;
Shu, Ching-Fong ;
Chi, Yun ;
Jen, Alex K. -Y. .
ADVANCED MATERIALS, 2009, 21 (03) :361-365
[9]   MULTILAYER WHITE LIGHT-EMITTING ORGANIC ELECTROLUMINESCENT DEVICE [J].
KIDO, J ;
KIMURA, M ;
NAGAI, K .
SCIENCE, 1995, 267 (5202) :1332-1334
[10]   White-light-emitting diodes based on iridium complexes via efficient energy transfer from a conjugated polymer [J].
Kim, TH ;
Lee, HK ;
Park, OO ;
Chin, BD ;
Lee, SH ;
Kim, JK .
ADVANCED FUNCTIONAL MATERIALS, 2006, 16 (05) :611-617