MOZART, a global chemical transport model for ozone and related chemical tracers 1. Model description

被引:356
作者
Brasseur, GP
Hauglustaine, DA
Walters, S
Rasch, PJ
Muller, JF
Granier, C
Tie, XX
机构
[1] Natl Ctr Atmospher Res, Boulder, CO 80307 USA
[2] Univ Paris 06, CNRS, Serv Aeron, F-75252 Paris 05, France
[3] Inst Aeron Spatiale Belgique, B-1180 Brussels, Belgium
[4] NOAA, Aeron Lab, Boulder, CO 80303 USA
[5] Univ Colorado, CIRES, Boulder, CO 80309 USA
关键词
D O I
10.1029/98JD02397
中图分类号
P4 [大气科学(气象学)];
学科分类号
0706 ; 070601 ;
摘要
We present a new global three-dimensional chemical-transport model (called MOZART) developed in the framework of the NCAR Community Climate Model (CCM) and aimed at studying the distribution and budget of tropospheric ozone and its precursors. The model, developed with a horizontal resolution of 2.8 degrees in longitude and latitude, includes 25 levels in the vertical between the Earth's surface and an upper boundary located at approximately 35 km altitude. In its present configuration the model calculates the global distribution of 56 chemical constituents with a timestep of 20 min, and accounts for surface emission and deposition, large-scale advective transport, subscale convective and boundary layer exchanges, chemical and photochemical transformations, as well as wet scavenging. Transport is simulated "off line" from CCM with dynamical variables provided every 3 hours from preestablished history tapes. Advection is calculated using the semi-Lagrangian transport scheme [Rasch and Williamson, 1990] developed for the MATCH model of Rasch et al. [1997]. Convective and boundary layer transports are expressed according to Hack [1994] and Holtslag and Boville [1993], respectively. A detailed evaluation of the model results is provided in a companion paper [Hauglustaine et al., this issue]. An analysis of the spatial and temporal variability in the chemical fields predicted by the model suggests that regional events such as summertime ozone episodes in polluted areas can be simulated by MOZART.
引用
收藏
页码:28265 / 28289
页数:25
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