Source tracing of chromium-, manganese-, nickel- and zinc-containing particles (PM10) by micro-PIXE spectrum

被引:20
作者
Yue, Weisheng [1 ]
Li, Xiaolin [1 ]
Liu, Jiangfeng [1 ]
Li, Yulan [1 ]
Zhang, Guilin [1 ]
Li, Yan [1 ]
机构
[1] Chinese Acad Sci, Inst Appl Phys, Shanghai 201800, Peoples R China
基金
中国国家自然科学基金;
关键词
AEROSOL-PARTICLES; SOURCE IDENTIFICATION; PARTICULATE MATTER; SHANGHAI CITY; POLLUTION; SINGLE; ASSOCIATION; ATMOSPHERE; MORTALITY; FINE;
D O I
10.1007/s10967-006-6896-y
中图分类号
O65 [分析化学];
学科分类号
070302 ; 081704 ;
摘要
Adverse health effects of occupational exposures to metal-containing airborne particles have long been recognized. To reduce the adverse effects caused by metal-containing particles, it is important to make clear where they are from. SPM has been applied to the study of the sources of chromium, manganese, nickel and zinc in aerosol particles PM10. Micro-PIXE spectra of single particles were treated as fingerprints since each particle was characterized by its micro-PIXE spectrum. The sources of the metal-containing particles were identified using the fingerprints of single particles. The study shows that the major sources of the four kinds of metals in the air are metallurgic emission, vehicle exhaust, coal combustion and soil dust.
引用
收藏
页码:115 / 121
页数:7
相关论文
共 21 条
[1]   Uptake and reduction of Cr(VI) to Cr(III) by mesquite (Prosopis spp.):: Chromate-plant interaction in hydroponics and solid media studied using XAS [J].
Aldrich, MV ;
Gardea-Torresdey, JL ;
Peralta-Videa, JR ;
Parsons, JG .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2003, 37 (09) :1859-1864
[2]   Micro-PIXE and principal component analysis in a study of internal mixing phenomena in Antarctic coastal aerosol [J].
Biancato, D. ;
Ceccato, D. ;
Chiminello, F. ;
Mittner, P. .
NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS, 2006, 249 :561-565
[3]   AN ASSOCIATION BETWEEN AIR-POLLUTION AND MORTALITY IN 6 UNITED-STATES CITIES [J].
DOCKERY, DW ;
POPE, CA ;
XU, XP ;
SPENGLER, JD ;
WARE, JH ;
FAY, ME ;
FERRIS, BG ;
SPEIZER, FE .
NEW ENGLAND JOURNAL OF MEDICINE, 1993, 329 (24) :1753-1759
[4]   Formation and chemical speciation of arsenic-, chromium-, and nickel-bearing coal combustion PM2.5 [J].
Galbreath, KC ;
Zygarlicke, CJ .
FUEL PROCESSING TECHNOLOGY, 2004, 85 (6-7) :701-726
[5]  
Jie Z, 1999, INTERNET TESL J, V5
[6]   Pulmonary responses to oil fly ash particles in the rat differ by virtue of their specific soluble metals [J].
Kodavanti, UP ;
Hauser, R ;
Christiani, DC ;
Meng, ZH ;
McGee, J ;
Ledbetter, A ;
Richards, J ;
Costa, DL .
TOXICOLOGICAL SCIENCES, 1998, 43 (02) :204-212
[7]   Association of fine particulate matter from different sources with daily mortality in six US cities [J].
Laden, F ;
Neas, LM ;
Dockery, DW ;
Schwartz, J .
ENVIRONMENTAL HEALTH PERSPECTIVES, 2000, 108 (10) :941-947
[8]   Preliminary studies on the source of PM10 aerosol particles in the atmosphere of Shanghai City by analyzing single aerosol particles [J].
Li, X ;
Zhu, J ;
Guo, P ;
Wang, J ;
Qiu, Z ;
Lu, R ;
Qiu, H ;
Li, M ;
Jiang, D ;
Li, Y ;
Zhang, G .
NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS, 2003, 210 :412-417
[9]   A case study of the single and size-resolved particles in roadway tunnel in Seoul, Korea [J].
Ma, CJ ;
Tohno, S ;
Kasahara, M .
ATMOSPHERIC ENVIRONMENT, 2004, 38 (38) :6673-6677
[10]  
MALDERN HV, 2001, XRAY SPECTROM, V30, P320