Studies of third-order nonlinear optical properties of C60 by the optical Kerr effect

被引：12

作者：

Yung, MF ^{[1
]}

Wong, KY ^{[1
]}

机构：

[1] Chinese Univ Hong Kong, Dept Phys, Hong Kong, Peoples R China

来源：

APPLIED PHYSICS B-LASERS AND OPTICS | 1998年 / 66卷 / 05期

关键词：

D O I：

10.1007/s003400050439

中图分类号：

O43 [光学];

学科分类号：

070207 ; 0803 ;

摘要：

Second hyperpolarizability gamma of C-60 at 1.064 mu m is determined by the optical Kerr effect in toluene solution. Values of -6.5 x 10(-33) esu and 2.0 x 10(-32) esu for the real and imaginary parts of gamma, respectively, are obtained. Based on the experimental results and symmetry constraint, it is concluded that a three-level model is not adequate to describe the third-order nonlinearity of C-60. It is also inferred that the non-resonant gamma of C-60 should be positive in sign, which is in agreement with reported off-resonant measurements of gamma of C-60 by third-harmonic generation.

引用

页码：585 / 588

页数：4

共 22 条

[1] 3RD-ORDER NONLINEAR-OPTICAL INTERACTIONS OF C-60 AND C-70 [J].

ARANDA, FJ ;

RAO, DVGLN ;

ROACH, JF ;

TAYEBATI, P .

JOURNAL OF APPLIED PHYSICS, 1993, 73 (11) :7949-7951

[2] LARGE INFRARED NONLINEAR OPTICAL-RESPONSE OF C60 [J].

BLAU, WJ ;

BYRNE, HJ ;

CARDIN, DJ ;

DENNIS, TJ ;

HARE, JP ;

KROTO, HW ;

TAYLOR, R ;

WALTON, DRM .

PHYSICAL REVIEW LETTERS, 1991, 67 (11) :1423-1425

[3] Measurement of the resonant third-order nonlinear susceptibility of C-60 by nondegenerate four-wave mixing [J].

Geng, L ;

Wright, JC .

CHEMICAL PHYSICS LETTERS, 1996, 249 (1-2) :105-111

[4] NONRESONANT 3RD-ORDER OPTICAL NONLINEARITY OF ALL-CARBON MOLECULES C-60 [J].

GONG, QH ;

SUN, YX ;

XIA, ZJ ;

ZOU, YH ;

GU, ZN ;

ZHOU, XH ;

DI, Q .

JOURNAL OF APPLIED PHYSICS, 1992, 71 (06) :3025-3026

[5] NONLINEAR OPTICAL-PROPERTIES OF LINEAR-CHAINS AND ELECTRON-CORRELATION EFFECTS [J].

HEFLIN, JR ;

WONG, KY ;

ZAMANIKHAMIRI, O ;

GARITO, AF .

PHYSICAL REVIEW B, 1988, 38 (02) :1573-1576

[6] OPTICAL 2ND-HARMONIC AND 3RD-HARMONIC GENERATIONS IN C-60 FILM [J].

HOSHI, H ;

NAKAMURA, N ;

MARUYAMA, Y ;

NAKAGAWA, T ;

SUZUKI, S ;

SHIROMARU, H ;

ACHIBA, Y .

JAPANESE JOURNAL OF APPLIED PHYSICS PART 2-LETTERS & EXPRESS LETTERS, 1991, 30 (8A) :L1397-L1398

[7] OFF-RESONANT NONLINEAR OPTICAL-PROPERTIES OF C60 STUDIED BY DEGENERATE 4-WAVE-MIXING [J].

KAFAFI, ZH ;

LINDLE, JR ;

PONG, RGS ;

BARTOLI, FJ ;

LINGG, LJ ;

MILLIKEN, J .

CHEMICAL PHYSICS LETTERS, 1992, 188 (5-6) :492-496

[8]

KAFAFI ZH, 1992, PHYS REV LETT, V68, P2705, DOI 10.1103/PhysRevLett.68.2705

[9] NONLINEAR OPTICAL-PROPERTIES OF SUBLIMED C-60 THIN-FILMS [J].

KAJZAR, F ;

TALIANI, C ;

ZAMBONI, R ;

ROSSINI, S ;

DANIELI, R .

SYNTHETIC METALS, 1993, 54 (1-3) :21-32

[10] LARGE INFRARED NONLINEAR OPTICAL-RESPONSE OF C-60 - COMMENT [J].

KNIZE, RJ ;

PARTANEN, JP .

PHYSICAL REVIEW LETTERS, 1992, 68 (17) :2704-2704

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