Linear and nonlinear optical properties of BiFeO3

被引:218
作者
Kumar, Amit [1 ]
Rai, Ram C. [2 ]
Podraza, Nikolas J. [1 ]
Denev, Sava [1 ]
Ramirez, Mariola [1 ]
Chu, Ying-Hao [3 ]
Martin, Lane W. [3 ]
Ihlefeld, Jon [1 ]
Heeg, T. [4 ]
Schubert, J. [4 ]
Schlom, Darrell G. [1 ]
Orenstein, J. [5 ]
Ramesh, R. [3 ]
Collins, Robert W. [6 ]
Musfeldt, Janice L. [2 ]
Gopalan, Venkatraman [1 ]
机构
[1] Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA
[2] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA
[3] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA
[4] Inst Bio & Nano Syst, Res Ctr Julich, D-52425 Julich, Germany
[5] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA
[6] Univ Toledo, Dept Phys & Astron, Toledo, OH 43606 USA
基金
美国国家科学基金会;
关键词
D O I
10.1063/1.2901168
中图分类号
O59 [应用物理学];
学科分类号
摘要
Using spectroscopic ellipsometry, the room temperature refractive index and absorption versus wavelength of the ferroelectric antiferromagnet bismuth ferrite, BiFeO3, are reported. The material has a direct band gap at 442 nm wavelength (2.81 eV). Using optical second harmonic generation, the nonlinear optical coefficients were determined to be d(15)/d(22)=0.20 +/- 0.01, d(31)/d(22) = 0.35 +/- 0.02, d(33)/d(22)=-11.4 +/- 0.20, and vertical bar d(22)vertical bar = 298.4 +/- 6.1 pm/V at a fundamental wavelength of 800 nm. (C) 2008 American Institute of Physics.
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页数:3
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