Efficient non-fullerene polymer solar cells enabled by tetrahedron-shaped core based 3D-structure small-molecular electron acceptors

被引：99

作者：

Liu, Yuhang ^{[1
,2
,3
,4
]}

Lai, Joshua Yuk Lin ^{[2
]}

Chen, Shangshang ^{[2
]}

Li, Yunke ^{[2
]}

Jiang, Kui ^{[1
,2
]}

Zhao, Jingbo ^{[2
]}

Li, Zhengke ^{[2
]}

Hu, Huawei ^{[2
,3
,4
]}

Ma, Tingxuan ^{[2
,3
,4
]}

Lin, Haoran ^{[2
]}

Liu, Jing ^{[2
]}

Zhang, Jie ^{[5
]}

Huang, Fei ^{[5
]}

Yu, Demei ^{[3
,4
]}

Yan, He ^{[1
,2
]}

机构：

[1] Hong Kong Univ Sci & Technol, Shenzhen Res Inst, Shenzhen 518057, Peoples R China

[2] Hong Kong Univ Sci & Technol, Dept Chem, Hong Kong, Hong Kong, Peoples R China

[3] Xi An Jiao Tong Univ, Joint Sch Sustainable Dev, Xian 710049, Peoples R China

[4] Xi An Jiao Tong Univ, MOE, Key Lab Nonequilibrium Synth & Modulat Condensed, Xian 710049, Peoples R China

[5] S China Univ Technol, State Key Lab Luminescent Mat & Devices, Inst Optoelect Mat & Devices, Guangzhou 510640, Guangdong, Peoples R China

来源：

JOURNAL OF MATERIALS CHEMISTRY A | 2015年 / 3卷 / 26期

基金：

美国国家科学基金会;

关键词：

PHOTOVOLTAIC CELLS; PERFORMANCE; FILM; AGGREGATION;

D O I：

10.1039/c5ta03093e

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

Here we report a series of tetraphenyl carbon-group (tetraphenylmethane (TPC), tetraphenylsilane (TPSi) and tetraphenylgermane (TPGe)) core based 3D-structure non-fullerene electron acceptors, enabling efficient polymer solar cells with a power conversion efficiency (PCE) of up to similar to 4.3%. The results showthat TPC and TPSi corebased polymer solar cells (PSCs) perform significantly better than that based on TPGe. Our study provides a new approach for designing small molecular acceptor materials for polymer solar cells.

引用

页码：13632 / 13636

页数：5

共 35 条

[31] Rylene and Related Diimides for Organic Electronics [J].

Zhan, Xiaowei ;

Facchetti, Antonio ;

Barlow, Stephen ;

Marks, Tobin J. ;

Ratner, Mark A. ;

Wasielewski, Michael R. ;

Marder, Seth R. .

ADVANCED MATERIALS, 2011, 23 (02) :268-284

[32] Non-Fullerene Organic Solar Cells with 6.1% Efficiency through Fine-Tuning Parameters of the Film-Forming Process [J].

Zhang, Xin ;

Zhan, Chuanlang ;

Yao, Jiannian .

CHEMISTRY OF MATERIALS, 2015, 27 (01) :166-173

[33] A Potential Perylene Diimide Dimer-Based Acceptor Material for Highly Efficient Solution-Processed Non-Fullerene Organic Solar Cells with 4.03% Efficiency [J].

Zhang, Xin ;

Lu, Zhenhuan ;

Ye, Long ;

Zhan, Chuanlang ;

Hou, Jianhui ;

Zhang, Shaoqing ;

Jiang, Bo ;

Zhao, Yan ;

Huang, Jianhua ;

Zhang, Shanlin ;

Liu, Yang ;

Shi, Qiang ;

Liu, Yunqi ;

Yao, Jiannian .

ADVANCED MATERIALS, 2013, 25 (40) :5791-+

[34] High-efficiency non-fullerene organic solar cells enabled by a difluorobenzothiadiazole-based donor polymer combined with a properly matched small molecule acceptor [J].

Zhao, Jingbo ;

Li, Yunke ;

Lin, Haoran ;

Liu, Yuhang ;

Jiang, Kui ;

Mu, Cheng ;

Ma, Tingxuan ;

Lai, Joshua Yuk Lin ;

Hu, Huawei ;

Yu, Demei ;

Yan, He .

ENERGY & ENVIRONMENTAL SCIENCE, 2015, 8 (02) :520-525

[35] Microcavity-Enhanced Light-Trapping for Highly Efficient Organic Parallel Tandem Solar Cells [J].

Zuo, Lijian ;

Chueh, Chu-Chen ;

Xu, Yun-Xiang ;

Chen, Kung-Shih ;

Zang, Yue ;

Li, Chang-Zhi ;

Chen, Hongzheng ;

Jen, Alex K-Y .

ADVANCED MATERIALS, 2014, 26 (39) :6778-6784

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