Phonon-assisted excitonic recombination channels observed in DNA-wrapped carbon nanotubes using photoluminescence spectroscopy

被引:106
作者
Chou, SG [1 ]
Plentz, F
Jiang, J
Saito, R
Nezich, D
Ribeiro, HB
Jorio, A
Pimenta, MA
Samsonidze, GG
Santos, AP
Zheng, M
Onoa, GB
Semke, ED
Dresselhaus, G
Dresselhaus, MS
机构
[1] MIT, Dept Chem, Cambridge, MA 02139 USA
[2] Univ Fed Minas Gerais, Dept Fis, BR-30123970 Belo Horizonte, MG, Brazil
[3] Tohoku Univ, Dept Phys, Sendai, Miyagi 9808578, Japan
[4] CREST JST, Sendai, Miyagi 9808578, Japan
[5] MIT, Dept Phys, Cambridge, MA 02139 USA
[6] MIT, Dept Elect Engn & Comp Sci, Cambridge, MA 02139 USA
[7] CDTN CNEN, Ctr Desenvolvimento Tecn Nucl, BR-30123970 Belo Horizonte, MG, Brazil
[8] DuPont Co Inc, Cent Res & Dev, Expt Stn, Wilmington, DE 19880 USA
[9] MIT, Francis Bitter Natl Magnet Lab, Cambridge, MA 02139 USA
关键词
D O I
10.1103/PhysRevLett.94.127402
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
By using a sample of DNA-wrapped single-wall carbon nanotubes strongly enriched in the (6,5) nanotube, photoluminescence emissions observed at special excitation energy values were identified with specific mechanisms of phonon-assisted excitonic absorption and recombination processes associated with (6,5) nanotubes, including one-phonon, two-phonon, and some continuous-luminescence processes. Such detailed processes are not separately identified in three-dimensional semiconducting materials. A general theoretical framework is presented to interpret the experimentally observed phonon-assisted processes in terms of excitonic states.
引用
收藏
页码:1 / 4
页数:4
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