Dimethylsulfide oxidation and the ratio of methanesulfonate to non sea-salt sulfate in the marine aerosol

被引:48
作者
Ayers, GP
Cainey, JM
Granek, H
Leck, C
机构
[1] UNIV STOCKHOLM,DEPT METEOROL,S-10691 STOCKHOLM,SWEDEN
[2] MONASH UNIV,GIPPSLAND CTR ENVIRONM SCI,CHURCHILL,AUSTRALIA
关键词
DMS oxidation; marine aerosol; box model; cloud condensation nuclei; non sea-salt sulfate;
D O I
10.1007/BF00053798
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
A box model of DMS oxidation in the clean, low-NO, marine atmospheric boundary layer has been used to predict the latitude dependence of the aerosol methanesulfonate to non sea-salt sulfate ratio. The observed latitude dependence of this ratio in the Southern Hemisphere can be reproduced reasonably well if the full suite of reactions proposed by Yin ct al. (1990a) is employed, and a strong temperature dependence is specified in the rates of decomposition of CH3SO2 and CH3SO3 radicals.
引用
收藏
页码:307 / 325
页数:19
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