Aerosol direct radiative forcing over Djougou (northern Benin) during the African Monsoon Multidisciplinary Analysis dry season experiment (Special Observation Period-0)

被引:36
作者
Mallet, M. [1 ]
Pont, V. [1 ]
Liousse, C. [1 ]
Gomes, L. [2 ]
Pelon, J. [3 ]
Osborne, S. [4 ]
Haywood, J. [4 ]
Roger, J. C. [5 ]
Dubuisson, P. [6 ]
Mariscal, A. [1 ]
Thouret, V. [1 ]
Goloub, P. [7 ]
机构
[1] CNRS, UPS, UMR5560, Lab Aerol, F-31400 Toulouse, France
[2] CNRM, F-31057 Toulouse, France
[3] Univ Jussieu, Serv Aeron, F-75252 Paris 05, France
[4] Met Off, Exeter EX1 3PB, Devon, England
[5] OPGC, LAMP, F-63177 Clermont Ferrand, France
[6] ELICO, LOCL MREN, F-62930 Wimereux, France
[7] USTL, CNRS, Opt Atmospher Lab, F-59655 Lille, France
关键词
D O I
10.1029/2007JD009419
中图分类号
P4 [大气科学(气象学)];
学科分类号
0706 ; 070601 ;
摘要
The purpose of this work is to investigate the direct radiative forcing of aerosols over the supersite of Djougou (northern Benin) during the African Monsoon Multidisciplinary Analyses dry season experiment. We focus our simulations on the top of atmosphere, bottom of atmosphere, and atmosphere radiative forcings. During the dry season period, Sun photometer measurements indicate a rather turbid atmosphere with a mean aerosol optical depth for the overall period of 0.78 +/- 0.24 (at 440 nm). The aerosol absorption coefficient estimated at the surface ranged between 2.3 and 37.3 Mm(-1) (mean value 15.2 +/- 10.6 Mm(-1) at 520 nm) and the scattering coefficient between 44.5 and 232.3 Mm(-1) (mean 145 +/- 59 Mm(-1) at 520 nm). This leads to a single scattering albedo of between 0.81 and 0.98 (at 520 nm) with a mean (and standard deviation) value of 0.91 +/- 0.05, indicating moderately absorbing aerosols. In parallel, micropulse lidar measurements indicate the presence of two distinct aerosol layers, with a first one located between the surface and 1 km and a second one located above 1.5-4.0 km. On the basis of surface and aircraft observations, sunphotometer measurements, lidar profiles, and Moderate Resolution Imagaing Spectroradiometer sensor an estimation of the daily clear sky direct radiative forcing has been estimated for the 17 - 24 January 2006 period. Simulations indicate that aerosols reduce significantly the solar energy reaching the surface (mean Delta F-BOA = -61.5 W/m(2)) by reflection to space (mean Delta F-TOA = -18.4 W/m(2)) but predominantly by absorption of the solar radiation into the atmosphere (mean Delta F-ATM = +43.1 W/m(2)). The mean heating rate at the surface and within the elevated biomass burning layer is considerably enhanced by 1.50 and 1.90 K day(-1), respectively.
引用
收藏
页数:16
相关论文
共 63 条
[1]   The direct radiative effect of biomass burning aerosols over southern Africa [J].
Abel, SJ ;
Highwood, EJ ;
Haywood, JM ;
Stringer, MA .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2005, 5 :1999-2018
[2]   Reduction of tropical cloudiness by soot [J].
Ackerman, AS ;
Toon, OB ;
Stevens, DE ;
Heymsfield, AJ ;
Ramanathan, V ;
Welton, EJ .
SCIENCE, 2000, 288 (5468) :1042-1047
[3]   Chemical and optical characterization of aerosols measured in spring 2002 at the ACE-Asia supersite, Zhenbeitai, China [J].
Alfaro, SC ;
Gomes, L ;
Rajot, JL ;
Lafon, S ;
Gaudichet, A ;
Chatenet, B ;
Maille, M ;
Cautenet, G ;
Lasserre, F ;
Cachier, H ;
Zhang, XY .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2003, 108 (D23)
[4]   Variability of aerosol optical properties derived from in situ aircraft measurements during ACE-Asia [J].
Anderson, TL ;
Masonis, SJ ;
Covert, DS ;
Ahlquist, NC ;
Howell, SG ;
Clarke, AD ;
McNaughton, CS .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2003, 108 (D23)
[5]   Determining aerosol radiative properties using the TSI 3563 integrating nephelometer [J].
Anderson, TL ;
Ogren, JA .
AEROSOL SCIENCE AND TECHNOLOGY, 1998, 29 (01) :57-69
[6]   Estimating the direct aerosol radiative perturbation:: Impact of ocean surface representation and aerosol non-sphericity [J].
Bellouin, N ;
Boucher, O ;
Vesperini, M ;
Tanré, D .
QUARTERLY JOURNAL OF THE ROYAL METEOROLOGICAL SOCIETY, 2004, 130 (601) :2217-2232
[7]   Aerosol optical properties at Sagres, Portugal during ACE-2 [J].
Carrico, CM ;
Rood, MJ ;
Ogren, JA ;
Neusüss, C ;
Wiedensohler, A ;
Heintzenberg, J .
TELLUS SERIES B-CHEMICAL AND PHYSICAL METEOROLOGY, 2000, 52 (02) :694-715
[8]   Optical and physical properties of aerosols in the boundary layer and free troposphere over the Amazon Basin during the biomass burning season [J].
Chand, D. ;
Guyon, P. ;
Artaxo, P. ;
Schmid, O. ;
Frank, G. P. ;
Rizzo, L. V. ;
Mayol-Bracero, O. L. ;
Gatti, L. V. ;
Andreae, M. O. .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2006, 6 :2911-2925
[9]   Global anthropogenic aerosol direct forcing derived from satellite and ground-based observations [J].
Chung, CE ;
Ramanathan, V ;
Kim, D ;
Podgorny, IA .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2005, 110 (D24) :1-17
[10]   Accuracy assessments of aerosol optical properties retrieved from Aerosol Robotic Network (AERONET) Sun and sky radiance measurements [J].
Dubovik, O ;
Smirnov, A ;
Holben, BN ;
King, MD ;
Kaufman, YJ ;
Eck, TF ;
Slutsker, I .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2000, 105 (D8) :9791-9806