Aerosol direct radiative forcing over Djougou (northern Benin) during the African Monsoon Multidisciplinary Analysis dry season experiment (Special Observation Period-0)

被引:36
作者
Mallet, M. [1 ]
Pont, V. [1 ]
Liousse, C. [1 ]
Gomes, L. [2 ]
Pelon, J. [3 ]
Osborne, S. [4 ]
Haywood, J. [4 ]
Roger, J. C. [5 ]
Dubuisson, P. [6 ]
Mariscal, A. [1 ]
Thouret, V. [1 ]
Goloub, P. [7 ]
机构
[1] CNRS, UPS, UMR5560, Lab Aerol, F-31400 Toulouse, France
[2] CNRM, F-31057 Toulouse, France
[3] Univ Jussieu, Serv Aeron, F-75252 Paris 05, France
[4] Met Off, Exeter EX1 3PB, Devon, England
[5] OPGC, LAMP, F-63177 Clermont Ferrand, France
[6] ELICO, LOCL MREN, F-62930 Wimereux, France
[7] USTL, CNRS, Opt Atmospher Lab, F-59655 Lille, France
关键词
D O I
10.1029/2007JD009419
中图分类号
P4 [大气科学(气象学)];
学科分类号
0706 ; 070601 ;
摘要
The purpose of this work is to investigate the direct radiative forcing of aerosols over the supersite of Djougou (northern Benin) during the African Monsoon Multidisciplinary Analyses dry season experiment. We focus our simulations on the top of atmosphere, bottom of atmosphere, and atmosphere radiative forcings. During the dry season period, Sun photometer measurements indicate a rather turbid atmosphere with a mean aerosol optical depth for the overall period of 0.78 +/- 0.24 (at 440 nm). The aerosol absorption coefficient estimated at the surface ranged between 2.3 and 37.3 Mm(-1) (mean value 15.2 +/- 10.6 Mm(-1) at 520 nm) and the scattering coefficient between 44.5 and 232.3 Mm(-1) (mean 145 +/- 59 Mm(-1) at 520 nm). This leads to a single scattering albedo of between 0.81 and 0.98 (at 520 nm) with a mean (and standard deviation) value of 0.91 +/- 0.05, indicating moderately absorbing aerosols. In parallel, micropulse lidar measurements indicate the presence of two distinct aerosol layers, with a first one located between the surface and 1 km and a second one located above 1.5-4.0 km. On the basis of surface and aircraft observations, sunphotometer measurements, lidar profiles, and Moderate Resolution Imagaing Spectroradiometer sensor an estimation of the daily clear sky direct radiative forcing has been estimated for the 17 - 24 January 2006 period. Simulations indicate that aerosols reduce significantly the solar energy reaching the surface (mean Delta F-BOA = -61.5 W/m(2)) by reflection to space (mean Delta F-TOA = -18.4 W/m(2)) but predominantly by absorption of the solar radiation into the atmosphere (mean Delta F-ATM = +43.1 W/m(2)). The mean heating rate at the surface and within the elevated biomass burning layer is considerably enhanced by 1.50 and 1.90 K day(-1), respectively.
引用
收藏
页数:16
相关论文
共 63 条
[41]   Simulation of aerosol radiative properties with the ORISAM-RAD model durin a pollution event (ESCOMPTE 2001) [J].
Mallet, M. ;
Pont, V. ;
Liousse, C. ;
Roger, J. C. ;
Dubuisson, P. .
ATMOSPHERIC ENVIRONMENT, 2006, 40 (40) :7696-7705
[42]   Carbonaceous aerosols over the Indian Ocean during the Indian Ocean Experiment (INDOEX): Chemical characterization, optical properties, and probable sources [J].
Mayol-Bracero, OL ;
Gabriel, R ;
Andreae, MO ;
Kirchstetter, TW ;
Novakov, T ;
Ogren, J ;
Sheridan, P ;
Streets, DG .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2002, 107 (D19)
[43]   Physical and optical properties of mineral dust aerosol during the Dust and Biomass-burning Experiment [J].
Osborne, S. R. ;
Johnson, B. T. ;
Haywood, J. M. ;
Baran, A. J. ;
Harrison, M. A. J. ;
McConnell, C. L. .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2008, 113
[44]   Vertical profiles of aerosol scattering and absorption measured in situ during the North Atlantic Aerosol Characterization Experiment (ACE-2) [J].
Öström, E ;
Noone, KJ .
TELLUS SERIES B-CHEMICAL AND PHYSICAL METEOROLOGY, 2000, 52 (02) :526-545
[45]   Microlidar observations of biomass burning aerosol over Djougou (Benin) during African Monsoon Multidisciplinary Analysis Special Observation Period 0: Dust and Biomass-Burning Experiment [J].
Pelon, J. ;
Mallet, M. ;
Mariscal, A. ;
Goloub, P. ;
Tanre, D. ;
Karam, D. Bou ;
Flamant, C. ;
Haywood, J. ;
Pospichal, B. ;
Victori, S. .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2008, 113 (D23)
[46]   The dependence of the specific attenuation cross-section on black carbon mass fraction and particle size [J].
Petzold, A ;
Kopp, C ;
Niessner, R .
ATMOSPHERIC ENVIRONMENT, 1997, 31 (05) :661-672
[47]   Multiyear analysis of amazonian biomass burning smoke radiative forcing of climate [J].
Procopio, AS ;
Artaxo, P ;
Kaufman, YJ ;
Remer, LA ;
Schafer, JS ;
Holben, BN .
GEOPHYSICAL RESEARCH LETTERS, 2004, 31 (03) :L031081-4
[48]   Chemical mass closure and assessment of the origin of the submicron aerosol in the marine boundary layer and the free troposphere at Tenerife during ACE-2 [J].
Putaud, JP ;
Van Dingenen, R ;
Mangoni, M ;
Virkkula, A ;
Raes, F ;
Maring, H ;
Prospero, JM ;
Swietlicki, E ;
Berg, OH ;
Hillamo, R ;
Mäkelä, T .
TELLUS SERIES B-CHEMICAL AND PHYSICAL METEOROLOGY, 2000, 52 (02) :141-168
[49]   A comparison of aerosol chemical and optical properties from the 1st and 2nd Aerosol Characterization Experiments [J].
Quinn, PK ;
Bates, TS ;
Coffman, DJ ;
Miller, TL ;
Johnson, JE ;
Covert, DS ;
Putaud, JP ;
Neusüss, C ;
Novakov, T .
TELLUS SERIES B-CHEMICAL AND PHYSICAL METEOROLOGY, 2000, 52 (02) :239-257
[50]   Indian Ocean Experiment: An integrated analysis of the climate forcing and effects of the great Indo-Asian haze [J].
Ramanathan, V ;
Crutzen, PJ ;
Lelieveld, J ;
Mitra, AP ;
Althausen, D ;
Anderson, J ;
Andreae, MO ;
Cantrell, W ;
Cass, GR ;
Chung, CE ;
Clarke, AD ;
Coakley, JA ;
Collins, WD ;
Conant, WC ;
Dulac, F ;
Heintzenberg, J ;
Heymsfield, AJ ;
Holben, B ;
Howell, S ;
Hudson, J ;
Jayaraman, A ;
Kiehl, JT ;
Krishnamurti, TN ;
Lubin, D ;
McFarquhar, G ;
Novakov, T ;
Ogren, JA ;
Podgorny, IA ;
Prather, K ;
Priestley, K ;
Prospero, JM ;
Quinn, PK ;
Rajeev, K ;
Rasch, P ;
Rupert, S ;
Sadourny, R ;
Satheesh, SK ;
Shaw, GE ;
Sheridan, P ;
Valero, FPJ .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2001, 106 (D22) :28371-28398