Conversion of CH4 and CO2 to syngas and higher hydrocarbons using dielectric barrier discharge

被引:25
作者
Hwang, BB
Yeo, YK [1 ]
Na, BK
机构
[1] Hanyang Univ, Dept Chem Engn, Seoul 133791, South Korea
[2] Korea Inst Sci & Technol, Clean Technol Ctr, Seoul 136791, South Korea
关键词
methane conversion; dielectric barrier discharge; syngas; electron energy distribution;
D O I
10.1007/BF02706899
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
The conversion of methane to syngas and other hydrocarbons in dielectric barrier discharge plasma under the presence of CO2 was investigated. Effects of the input voltage on the conversion of methane and CO, and the ratio of syngas were analyzed experimentally. The results of numerical simulations showed good quantitative agreement with those of experiments.
引用
收藏
页码:631 / 634
页数:4
相关论文
共 16 条
[1]  
Busch C, 2000, CONTRIB PLASM PHYS, V40, P81, DOI 10.1002/(SICI)1521-3986(200004)40:1/2<81::AID-CTPP81>3.0.CO
[2]  
2-7
[3]   The Fischer-Tropsch process: 1950-2000 [J].
Dry, ME .
CATALYSIS TODAY, 2002, 71 (3-4) :227-241
[4]   Direct conversion of methane and carbon dioxide to higher hydrocarbons using catalytic dielectric-barrier discharges with zeolites [J].
Eliasson, B ;
Liu, CJ ;
Kogelschatz, U .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2000, 39 (05) :1221-1227
[5]   Conversion of methane to higher hydrocarbons in pulsed DC barrier discharge at atmospheric pressure [J].
Jeong, HK ;
Kim, SC ;
Han, C ;
Lee, H ;
Song, HK ;
Na, BK .
KOREAN JOURNAL OF CHEMICAL ENGINEERING, 2001, 18 (02) :196-201
[6]   Co-generation of syngas and higher hydrocarbons from CO2 and CH4 using dielectric-barrier discharge:: Effect of electrode materials [J].
Li, Y ;
Xu, GH ;
Liu, CJ ;
Eliasson, B ;
Xue, BZ .
ENERGY & FUELS, 2001, 15 (02) :299-302
[7]   Methane conversion to higher hydrocarbons in the presence of carbon dioxide using dielectric-barrier discharge plasmas [J].
Liu, CJ ;
Xue, BZ ;
Eliasson, B ;
He, F ;
Li, Y ;
Xu, GH .
PLASMA CHEMISTRY AND PLASMA PROCESSING, 2001, 21 (03) :301-310
[8]   Different approaches for methane plasmas modeling [J].
Masi, M ;
Cavallotti, C ;
Carra, S .
CHEMICAL ENGINEERING SCIENCE, 1998, 53 (22) :3875-3886
[9]   Selective oxidation of methane to methanol and formaldehyde with nitrous oxide in a dielectric-barrier discharge - Plasma reactor [J].
Matsumoto, H ;
Tanabe, S ;
Okitsu, K ;
Hayashi, Y ;
Suib, SL .
JOURNAL OF PHYSICAL CHEMISTRY A, 2001, 105 (21) :5304-5308
[10]   Syngas in perspective [J].
Rostrup-Nielsen, JR .
CATALYSIS TODAY, 2002, 71 (3-4) :243-247