Two-dimensional spectroscopy at infrared and optical frequencies

被引:252
作者
Hochstrasser, Robin M. [1 ]
机构
[1] Univ Penn, Dept Chem, Philadelphia, PA 19104 USA
关键词
D O I
10.1073/pnas.0704079104
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
This Perspective on multidimensional spectroscopy in the optical and infrared spectral regions focuses on the principles and the scientific and technical challenges facing these new fields. The methods hold great promise for advances in the visualization of time-dependent structural changes in complex systems ranging from liquids to biological assemblies, new materials, and fundamental physical processes. The papers in this special feature on multidimensional spectroscopy in chemistry, physics, and biology are typical of many recent advances.
引用
收藏
页码:14190 / 14196
页数:7
相关论文
共 65 条
[1]   Dynamics of water probed with vibrational echo correlation spectroscopy [J].
Asbury, JB ;
Steinel, T ;
Kwak, K ;
Corcelli, SA ;
Lawrence, CP ;
Skinner, JL ;
Fayer, MD .
JOURNAL OF CHEMICAL PHYSICS, 2004, 121 (24) :12431-12446
[2]   Two-dimensional infrared spectroscopy of peptides by phase-controlled femtosecond vibrational photon echoes [J].
Asplund, MC ;
Zanni, MT ;
Hochstrasser, RM .
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2000, 97 (15) :8219-8224
[3]   Hydrogen bonding and Raman, IR, and 2D-IR spectroscopy of dilute HOD in liquid D2O [J].
Auer, B. ;
Kumar, R. ;
Schmidt, J. R. ;
Skinner, J. L. .
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2007, 104 (36) :14215-14220
[4]   Picosecond conformational transition and equilibration of a cyclic peptide [J].
Bredenbeck, J ;
Helbing, J ;
Sieg, A ;
Schrader, T ;
Zinth, W ;
Renner, C ;
Behrendt, R ;
Moroder, L ;
Wachtveitl, J ;
Hamm, P .
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2003, 100 (11) :6452-6457
[5]   Protein ligand migration mapped by nonequilibrium 2D-IR exchange spectroscopy [J].
Bredenbeck, Jens ;
Helbing, Jan ;
Nienhaus, Karin ;
Nienhaus, G. Ulrich ;
Hamm, Peter .
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2007, 104 (36) :14243-14248
[6]   Two-dimensional spectroscopy of electronic couplings in photosynthesis [J].
Brixner, T ;
Stenger, J ;
Vaswani, HM ;
Cho, M ;
Blankenship, RE ;
Fleming, GR .
NATURE, 2005, 434 (7033) :625-628
[7]   Transient 2D IR spectroscopy of ubiquitin unfolding dynamics [J].
Chung, Hoi Sung ;
Ganim, Ziad ;
Jones, Kevin C. ;
Tokmakoff, Andrei .
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2007, 104 (36) :14237-14242
[8]   Ultrafast memory loss and energy redistribution in the hydrogen bond network of liquid H2O [J].
Cowan, ML ;
Bruner, BD ;
Huse, N ;
Dwyer, JR ;
Chugh, B ;
Nibbering, ETJ ;
Elsaesser, T ;
Miller, RJD .
NATURE, 2005, 434 (7030) :199-202
[9]   Single-shot two-dimensional spectrometer [J].
DeCamp, MF ;
Tokmakoff, A .
OPTICS LETTERS, 2006, 31 (01) :113-115
[10]   Heterodyned fifth-order two-dimensional IR spectroscopy: Third-quantum states and polarization selectivity [J].
Ding, F ;
Fulmer, EC ;
Zanni, MT .
JOURNAL OF CHEMICAL PHYSICS, 2005, 123 (09)