Donor/Acceptor Indenoperylene Dye for Highly Efficient Organic Dye-Sensitized Solar Cells

被引：544

作者：

Yao, Zhaoyang ^{[1
,2
]}

Zhang, Min ^{[1
]}

Wu, Heng ^{[1
]}

Yang, Lin ^{[1
,2
]}

Li, Renzhi ^{[1
]}

Wang, Peng ^{[1
]}

机构：

[1] Chinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Polymer Phys & Chem, Changchun 130022, Peoples R China

[2] Univ Chinese Acad Sci, Beijing 100049, Peoples R China

来源：

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY | 2015年 / 137卷 / 11期

基金：

美国国家科学基金会;

关键词：

N-ANNULATED PERYLENE; CHARGE-TRANSFER DYNAMICS; NANOCRYSTALLINE TIO2; LIGHT-ABSORPTION; PHOTOVOLTAIC PERFORMANCES; RUTHENIUM SENSITIZER; RECOMBINATION; ELECTROLYTE; PORPHYRINS; DESIGN;

D O I：

10.1021/jacs.5b01537

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

An N-annulated indenoperylene electrondonor decorated with photochemically inactive segments is synthesized and further conjugated via triple bond with electron-acceptor benzothiadiazolylbenzoic acid for a metal-free donor/acceptor dye. Without use of any coadsorbate, the judiciously tailored indenoperylene dye achieves a high-power conversion efficiency of 12.5% under irradiance of 100 mW cm(-2) AM1.5G sunlight.

引用

收藏

页码：3799 / 3802

页数：4

相关论文

共 69 条

[11] A novel charge extraction method for the study of electron transport and interfacial transfer in dye sensitised nanocrystalline solar cells [J].

Duffy, NW ;

Peter, LM ;

Rajapakse, RMG ;

Wijayantha, KGU .

ELECTROCHEMISTRY COMMUNICATIONS, 2000, 2 (09) :658-662

[12] Intramolecular charge-transfer tuning of perylenes:: Spectroscopic features and performance in Dye-sensitized solar cells [J].

Edvinsson, Tomas ;

Li, Chen ;

Pschirer, Neil ;

Schoeneboom, Jan ;

Eickemeyer, Felix ;

Sens, Ruediger ;

Boschloo, Gerrit ;

Herrmann, Andreas ;

Muellen, Klaus ;

Hagfeldt, Anders .

JOURNAL OF PHYSICAL CHEMISTRY C, 2007, 111 (42) :15137-15140

[13] Characterization of nanostructured hybrid and organic solar cells by impedance spectroscopy [J].

Fabregat-Santiago, Francisco ;

Garcia-Belmonte, Germa ;

Mora-Sero, Ivan ;

Bisquert, Juan .

PHYSICAL CHEMISTRY CHEMICAL PHYSICS, 2011, 13 (20) :9083-9118

[14] Design of Organic Dyes and Cobalt Polypyridine Redox Mediators for High-Efficiency Dye-Sensitized Solar Cells [J].

Feldt, Sandra M. ;

Gibson, Elizabeth A. ;

Gabrielsson, Erik ;

Sun, Licheng ;

Boschloo, Gerrit ;

Hagfeldt, Anders .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2010, 132 (46) :16714-16724

[15] Dye sensitization of nanocrystalline tin oxide by perylene derivatives [J].

Ferrere, S ;

Zaban, A ;

Gregg, BA .

JOURNAL OF PHYSICAL CHEMISTRY B, 1997, 101 (23) :4490-4493

[16] New perylenes for dye sensitization of TiO2 [J].

Ferrere, S ;

Gregg, BA .

NEW JOURNAL OF CHEMISTRY, 2002, 26 (09) :1155-1160

[17] Synthesis of new perylene imide dyes and their photovoltaic performances in nanocrystalline TiO2 dye-sensitized solar cells [J].

Fortage, Jerome ;

Severac, Marjorie ;

Houarner-Rassin, Coralie ;

Pellegrin, Yann ;

Blart, Errol ;

Odobel, Fabrice .

JOURNAL OF PHOTOCHEMISTRY AND PHOTOBIOLOGY A-CHEMISTRY, 2008, 197 (2-3) :156-169

[18] Femtosecond Diffuse Reflectance Transient Absorption for Dye-Sensitized Solar Cells under Operational Conditions: Effect of Electrolyte on Electron Injection [J].

Furube, Akihiro ;

Wang, Zhong-Sheng ;

Sunahara, Kenji ;

Hara, Kohjiro ;

Katoh, Ryuzi ;

Tachiya, Masanori .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2010, 132 (19) :6614-+

[19] Enhance the optical absorptivity of nanocrystalline TiO2 film with high molar extinction coefficient ruthenium sensitizers for high performance dye-sensitized solar cells [J].

Gao, Feifei ;

Wang, Yuan ;

Shi, Dong ;

Zhang, Jing ;

Wang, Mingkui ;

Jing, Xiaoyan ;

Humphry-Baker, Robin ;

Wang, Peng ;

Zakeeruddin, Shaik M. ;

Graetzel, Michael .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2008, 130 (32) :10720-10728

[20] Porphyrins for dye-sensitised solar cells: new insights into efficiency-determining electron transfer steps [J].

Griffith, Matthew J. ;

Sunahara, Kenji ;

Wagner, Pawel ;

Wagner, Klaudia ;

Wallace, Gordon G. ;

Officer, David L. ;

Furube, Akihiro ;

Katoh, Ryuzi ;

Mori, Shogo ;

Mozer, Attila J. .

CHEMICAL COMMUNICATIONS, 2012, 48 (35) :4145-4162

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