Automated radioxenon monitoring for the comprehensive nuclear-test-ban treaty in two distinctive locations: Ottawa and Tahiti

被引:39
作者
Stocki, TJ
Blanchard, X
D'Amours, R
Ungar, RK
Fontaine, JP
Sohier, M
Bean, M
Taffary, T
Racine, J
Tracy, BL
Brachet, G
Jean, M
Meyerhof, D
机构
[1] Raidat Protect Bur, Ottawa, ON K1A 1C1, Canada
[2] CEA, F-91680 Bruyeres Le Chatel, France
[3] Canadian Meterol Ctr, Dorval, PQ H9P 1J3, Canada
关键词
SPALAX; comprehensive nuclear-test-ban treaty (CTBT) organisation; radioxenon monitoring; atmospheric modeling; xenon;
D O I
10.1016/j.jenvrad.2004.10.005
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
In preparation for verification of the Comprehensive Nuclear-Test-Ban-Treaty, automated radioxenon monitoring is performed in two distinctive environments: Ottawa and Tahiti. These site's are monitored with SPALAX (Systeme de Prelevement d'air Automatique en Ligne avec l'Analyse des radioXenons) technology, which automatically extracts radioxenon from the atmosphere and measures the activity concentrations of Xe-131m,Xe-133m,Xe-133,Xe-135. The resulting isotopic concentrations can be useful to discern nuclear explosions from nuclear industry xenon emissions. Ambient radon background, which may adversely impact analyser sensitivity, is discussed. Upper concentration limits are reported for the apparently radioxenon free Tahiti environment. Ottawa has a complex radioxenon background due to proximity to nuclear reactors and medical isotope facilities. Meteorological models suggest that, depending on the wind direction, the radioxenon detected in Ottawa can. be characteristic of the normal radioxenon background in the Eastern United States, Europe, and Japan or distinctive due to medical isotope production. (c) 2004 Elsevier Ltd. All rights reserved.
引用
收藏
页码:305 / 326
页数:22
相关论文
共 25 条
[1]  
[Anonymous], 1996, T AM NUCL SOC
[2]   Intercomparison experiments of systems for the measurement of xenon radionuclides in the atmosphere [J].
Auer, M ;
Axelsson, A ;
Blanchard, X ;
Bowyer, TW ;
Brachet, G ;
Bulowski, I ;
Dubasov, Y ;
Elmgren, K ;
Fontaine, JP ;
Harms, W ;
Hayes, JC ;
Heimbigner, TR ;
McIntyre, JI ;
Panisko, ME ;
Popov, Y ;
Ringbom, A ;
Sartorius, H ;
Schmid, S ;
Schulze, J ;
Schlosser, C ;
Taffary, T ;
Weisse, W ;
Wernsperger, B .
APPLIED RADIATION AND ISOTOPES, 2004, 60 (06) :863-877
[3]  
Bowyer T.W., 1998, ENCY ENV ANAL REMEDI, P5295
[4]   Detection and analysis of xenon isotopes for the comprehensive nuclear-test-ban treaty international monitoring system [J].
Bowyer, TW ;
Schlosser, C ;
Abel, KH ;
Auer, M ;
Hayes, JC ;
Heimbigner, TR ;
McIntyre, JI ;
Panisko, ME ;
Reeder, PL ;
Satorius, H ;
Schulze, J ;
Weiss, W .
JOURNAL OF ENVIRONMENTAL RADIOACTIVITY, 2002, 59 (02) :139-151
[5]   Ambient Xe-133 levels in the northeast US [J].
Bowyer, TW ;
Abel, KH ;
Hensley, WK ;
Panisko, ME ;
Perkins, RW .
JOURNAL OF ENVIRONMENTAL RADIOACTIVITY, 1997, 37 (02) :143-153
[6]   Automated separation and measurement of radioxenon for the Comprehensive Test Ban Treaty [J].
Bowyer, TW ;
Abel, KH ;
Hubbard, CW ;
McKinnon, AD ;
Panisko, ME ;
Perkins, RW ;
Reeder, PL ;
Thompson, RC ;
Warner, RA .
JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY, 1998, 235 (1-2) :77-81
[7]  
BOWYER TW, 1993, PNNL11424
[8]  
CANDU R, 2001, TN110701 ISR
[9]  
Collins J. T., 1978, Nuclear power waste technology, P167
[10]  
DEGEER LE, 1995, NATO ASI SERIES E, V303, P157