Statics and dynamics of incommensurate spin order in a geometrically frustrated antiferromagnet CdCr2O4 -: art. no. 247204

被引:145
作者
Chung, JH [1 ]
Matsuda, M
Lee, SH
Kakurai, K
Ueda, H
Sato, TJ
Takagi, H
Hong, KP
Park, S
机构
[1] Natl Inst Stand & Technol, NIST Ctr Neutron Res, Gaithersburg, MD 20899 USA
[2] Japan Atom Energy Res Inst, Adv Sci Res Ctr, Tokai, Ibaraki 3191195, Japan
[3] Univ Virginia, Dept Phys, Charlottesville, VA 22904 USA
[4] Univ Tokyo, Inst Solid State Phys, Kashiwa, Chiba 2778581, Japan
[5] Univ Tokyo, Grad Sch Frontier Sci, Kashiwa, Chiba 2778581, Japan
[6] Korea Atom Energy Res Inst, HANARO, Taejon, South Korea
关键词
D O I
10.1103/PhysRevLett.95.247204
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Using elastic and inelastic neutron scattering we show that a cubic spinel, CdCr2O4, undergoes an elongation along the c axis (c > a=b) at its spin-Peierls-like phase transition at T-N=7.8 K. The Neel phase (T < T-N) has an incommensurate spin structure with a characteristic wave vector Q(M)=(0,delta,1) with delta similar to 0.09 and with spins lying on the ac plane. This is in stark contrast to another well-known Cr-based spinel, ZnCr2O4, that undergoes a c-axis contraction and a commensurate spin order. The magnetic excitation of the incommensurate Neel state has a weak anisotropy gap of 0.6 meV and it consists of at least three bands extending up to 5 meV.
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