Sensitivity analysis of surface ozone to emission controls in Beijing and its neighboring area during the 2008 Olympic Games

被引:25
作者
Gao, Yi [1 ]
Zhang, Meigen [1 ]
机构
[1] Chinese Acad Sci, Inst Atmospher Phys, State Key Lab Atmospher Boundary Layer Phys & Atm, Beijing 100029, Peoples R China
基金
中国国家自然科学基金;
关键词
chemical smoke; tropospheric ozone; emission control; CMAQ; process analysis; AIR-QUALITY; TROPOSPHERIC OZONE; URBAN; TRANSPORT; EPISODES; ASIA;
D O I
10.1016/S1001-0742(11)60728-6
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The regional air quality modeling system RAMS (Regional Atmospheric Modeling System)-CMAQ (Community Multi-scale Air Quality modeling system) is applied to analyze temporal and spatial variations in surface ozone concentration over Beijing and its surrounding region from July to October 2008. Comparison of simulated and observed meteorological elements and concentration of nitrogen oxides (NOx) and ozone at one urban site and three rural sites during Olympic Games show that model can generally reproduce the main observed feature of wind, temperature and ozone, but NOx concentration is overestimated. Although ozone concentration decreased during Olympics, high ozone episodes occurred on 24 July and 24 August with concentration of 360 and 245 mu g/m(3) at Aoyuncun site, respectively. The analysis of sensitive test, with and without emission controls, shows that emission controls could reduce ozone concentration in the afternoon when ozone concentration was highest but increase it at night and in the morning. The evolution of the weather system during the ozone episodes (24 July and 24 August) indicates that hot and dry air and a stable weak pressure field intensified the production of ozone and allowed it to accumulate. Process analysis at the urban site and rural site shows that under favorable weather condition on 24 August, horizontal transport was the main contributor of the rural place and the pollution from the higher layer would be transported to the surface layer. On 24 July, as the wind velocity was smaller, the impact of transport on the rural place was not obvious.
引用
收藏
页码:50 / 61
页数:12
相关论文
共 32 条
[31]   A numerical study of tropospheric ozone in the springtime in East Asia [J].
Zhang, MG ;
Xu, YF ;
Uno, I ;
Akimoto, H .
ADVANCES IN ATMOSPHERIC SCIENCES, 2004, 21 (02) :163-170
[32]  
张远航, 1998, [北京大学学报. 自然科学版, Acta Scientiarum Naturalium Universitatis Pekinensis], V34, P392