Rotationally inelastic scattering of C2H2 from LiF(100): Translational energy dependence

被引:34
作者
Francisco, TW
Camillone, N
Miller, RE
机构
[1] Department of Chemistry, The University of North Carolina at Chapel Hill, Chapel Hill, NC
关键词
D O I
10.1103/PhysRevLett.77.1402
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We report the first results from a new experimental apparatus designed for the general investigation of energy transfer in molecule-surface scattering. The translational energy dependence of the rotational temperature of C2H2 scattered from LiF(100) has been measured, yielding results which are different from any data of this type previously reported. Our preliminary interpretation of the results is in terms of vibrational excitation with increasing incident translational energy.
引用
收藏
页码:1402 / 1405
页数:4
相关论文
共 26 条
[11]   DIRECT-INELASTIC AND TRAPPING-DESORPTION SCATTERING OF N-2 AND CH4 FROM PT(111) [J].
JANDA, KC ;
HURST, JE ;
COWIN, J ;
WHARTON, L ;
AUERBACH, DJ .
SURFACE SCIENCE, 1983, 130 (02) :395-409
[12]   OBSERVATION OF DIRECT MULTIQUANTUM VIBRATIONAL-EXCITATION IN GAS-SURFACE SCATTERING - NH3 ON AU(111) [J].
KAY, BD ;
RAYMOND, TD ;
COLTRIN, ME .
PHYSICAL REVIEW LETTERS, 1987, 59 (24) :2792-2794
[13]   ROTATIONAL ENERGY-TRANSFER IN DIRECT INELASTIC SURFACE SCATTERING - NO ON AG(111) [J].
KLEYN, AW ;
LUNTZ, AC ;
AUERBACH, DJ .
PHYSICAL REVIEW LETTERS, 1981, 47 (16) :1169-1172
[14]   DIRECT INELASTIC-SCATTERING OF NITRIC-OXIDE FROM CLEAN AG(111) - ROTATIONAL AND FINE-STRUCTURE DISTRIBUTIONS [J].
KUBIAK, GD ;
HURST, JE ;
RENNAGEL, HG ;
MCCLELLAND, GM ;
ZARE, RN .
JOURNAL OF CHEMICAL PHYSICS, 1983, 79 (10) :5163-5178
[15]   DIRECT INELASTIC-SCATTERING OF N-2 FROM AG(111) .4. SCATTERING FROM HIGH-TEMPERATURE SURFACE [J].
KUMMEL, AC ;
SITZ, GO ;
ZARE, RN ;
TULLY, JC .
JOURNAL OF CHEMICAL PHYSICS, 1989, 91 (09) :5793-5801
[16]  
Levine R.D., 1987, MOL REACTION DYNAMIC
[17]   ROTATIONALLY INELASTIC GAS-SURFACE SCATTERING - HCL FROM AU(111) [J].
LYKKE, KR ;
KAY, BD .
JOURNAL OF CHEMICAL PHYSICS, 1990, 92 (04) :2614-2623
[18]   DISTRIBUTION OF INTERNAL ENERGY IN CO AND CO2 VIBRATIONALLY EXCITED BY A HOT PLATINUM SURFACE [J].
MANTELL, DA ;
RYALI, SB ;
HALLER, GL ;
FENN, JB .
JOURNAL OF CHEMICAL PHYSICS, 1983, 78 (06) :4250-4255
[19]   DETERMINATION OF INTERNAL-STATE DISTRIBUTIONS OF SURFACE SCATTERED MOLECULES - INCOMPLETE ROTATIONAL ACCOMMODATION OF NO ON AG(111) [J].
MCCLELLAND, GM ;
KUBIAK, GD ;
RENNAGEL, HG ;
ZARE, RN .
PHYSICAL REVIEW LETTERS, 1981, 46 (13) :831-834
[20]   STATE-TO-STATE MOLECULAR-BEAM SCATTERING OF VIBRATIONALLY EXCITED NO FROM CLEAVED LIF(100) SURFACES [J].
MISEWICH, J ;
ZACHARIAS, H ;
LOY, MMT .
PHYSICAL REVIEW LETTERS, 1985, 55 (18) :1919-1922