One-dimensional transport with dynamic disorder

被引:4
作者
Barsegov, V [1 ]
Shapir, Y
Mukamel, S
机构
[1] Univ Rochester, Dept Chem, Rochester, NY 14627 USA
[2] Univ Rochester, Dept Phys & Astron, Rochester, NY 14627 USA
来源
PHYSICAL REVIEW E | 2003年 / 68卷 / 01期
关键词
D O I
10.1103/PhysRevE.68.011101
中图分类号
O35 [流体力学]; O53 [等离子体物理学];
学科分类号
070204 ; 080103 ; 080704 ;
摘要
We study the mean quenching time distribution and its moments in a one-dimensional N-site donor-bridge-acceptor system where all sites are coupled to a two-state jump bath for arbitrary disorder and an arbitrary ratio kappa=<k>/R of the bath jump rate R and the average hopping rate <k>. When kappaNsimilar to1, the quenching time distribution has long power-law tails even when the waiting times are exponentially distributed. These disappear for kappaN<<1 where the hopping rate self-averages on the bath relaxation time scale. In the absence of disorder or for small kappa, the mean quenching time scales linearly with N. Otherwise, we observe a power law, similar toN(1+gamma), with a crossover to linear scaling (gamma=0) for large N. Distributions of particle position, its second moment, velocity and diffusion coefficient are computed in the infinite N limit. For times longer than R-1, the dynamic disorder self-averages and the average position, velocity, and diffusion coefficient scale linearly in time.
引用
收藏
页码:14 / 111011
页数:14
相关论文
共 78 条
[61]   SPECTROSCOPY OF A CHROMOPHORE COUPLED TO A LATTICE OF DYNAMIC 2-LEVEL SYSTEMS .2. SPECTRAL DIFFUSION KERNEL [J].
REILLY, PD ;
SKINNER, JL .
JOURNAL OF CHEMICAL PHYSICS, 1994, 101 (02) :965-973
[62]   THE MEMBRANE SKELETON OF ERYTHROCYTES - A PERCOLATION MODEL [J].
SAXTON, MJ .
BIOPHYSICAL JOURNAL, 1990, 57 (06) :1167-1177
[63]   THE SPECTRIN NETWORK AS A BARRIER TO LATERAL DIFFUSION IN ERYTHROCYTES - A PERCOLATION ANALYSIS [J].
SAXTON, MJ .
BIOPHYSICAL JOURNAL, 1989, 55 (01) :21-28
[64]   SINGLE-PARTICLE TRACKING - EFFECTS OF CORRALS [J].
SAXTON, MJ .
BIOPHYSICAL JOURNAL, 1995, 69 (02) :389-398
[65]   Statistical analyses and theoretical models of single-molecule enzymatic dynamics [J].
Schenter, GK ;
Lu, HP ;
Xie, XS .
JOURNAL OF PHYSICAL CHEMISTRY A, 1999, 103 (49) :10477-10488
[66]   STOCHASTIC TRANSPORT IN A DISORDERED SOLID .2. IMPURITY CONDUCTION [J].
SCHER, H ;
LAX, M .
PHYSICAL REVIEW B, 1973, 7 (10) :4502-4519
[67]   STOCHASTIC TRANSPORT IN A DISORDERED SOLID .1. THEORY [J].
SCHER, H ;
LAX, M .
PHYSICAL REVIEW B, 1973, 7 (10) :4491-4502
[68]   ANOMALOUS TRANSIT-TIME DISPERSION IN AMORPHOUS SOLIDS [J].
SCHER, H ;
MONTROLL, EW .
PHYSICAL REVIEW B, 1975, 12 (06) :2455-2477
[69]   LATERAL MOBILITY OF INTEGRAL MEMBRANE-PROTEINS IS INCREASED IN SPHEROCYTIC ERYTHROCYTES [J].
SHEETZ, MP ;
SCHINDLER, M ;
KOPPEL, DE .
NATURE, 1980, 285 (5765) :510-512
[70]   ASYMPTOTIC SOLUTIONS OF CONTINUOUS-TIME RANDOM-WALKS [J].
SHLESING.MF .
JOURNAL OF STATISTICAL PHYSICS, 1974, 10 (05) :421-434