Direct measurement of rotationally inelastic cross sections at astrophysical and quantum collisional temperatures

被引:27
作者
Ball, CD [1 ]
De Lucia, FC [1 ]
机构
[1] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA
关键词
D O I
10.1103/PhysRevLett.81.305
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
The first measurements of rotationally inelastic collision cross sections over the 1-40 K temperature range characteristic of much of the interstellar medium are reported. Measurements of the 1(1,0)-1(0,1) transition of H2S in collision with He are based on a collisional cooling methodology, which allows the direct observation of collision processes at temperatures far below the limits ordinarily imposed by vapor pressure. These cross sections are also of fundamental interest because resonant formation of quasibound complexes mediates rotational energy transfer at low collision energy. [S0031-9007(98)06538-7].
引用
收藏
页码:305 / 308
页数:4
相关论文
共 20 条
[11]   Total and state-to-state rate coefficients for rotational energy transfer in collisions between NO(Chi(2)Pi) and He at temperatures down to 15 K [J].
James, PL ;
Sims, IR ;
Smith, IWM .
CHEMICAL PHYSICS LETTERS, 1997, 272 (5-6) :412-418
[12]   IMPROVED MODELING OF ATOM MOLECULE POTENTIAL-ENERGY SURFACES - ILLUSTRATIVE APPLICATION TO HE-CO [J].
LEROY, RJ ;
BISSONNETTE, C ;
WU, TH ;
DHAM, AK ;
MEATH, WJ .
FARADAY DISCUSSIONS, 1994, 97 :81-94
[13]  
MCGURK JC, 1974, ADV CHEM PHYS, V25, P1
[14]   MEASUREMENT OF PRESSURE-BROADENING PARAMETERS FOR THE CO-HE SYSTEM AT 4-K [J].
MESSER, JK ;
DELUCIA, FC .
PHYSICAL REVIEW LETTERS, 1984, 53 (27) :2555-2558
[15]   EFFECT OF THE POTENTIAL WELL ON LOW-TEMPERATURE PRESSURE BROADENING IN CO-HE [J].
PALMA, A ;
GREEN, S .
JOURNAL OF CHEMICAL PHYSICS, 1986, 85 (03) :1333-1335
[16]   PRESSURE BROADENING OF GAS-PHASE MOLECULAR-IONS AT VERY-LOW TEMPERATURE [J].
PEARSON, JC ;
OESTERLING, LC ;
HERBST, E ;
DELUCIA, FC .
PHYSICAL REVIEW LETTERS, 1995, 75 (16) :2940-2943
[17]   AB-INITIO POTENTIAL-ENERGY SURFACE AND DYNAMICS OF HE-CO [J].
TAO, FM ;
DRUCKER, S ;
COHEN, RC ;
KLEMPERER, W .
JOURNAL OF CHEMICAL PHYSICS, 1994, 101 (10) :8680-8686
[18]   TRANSIENT NUTATIONS IN NUCLEAR MAGNETIC RESONANCE [J].
TORREY, HC .
PHYSICAL REVIEW, 1949, 76 (08) :1059-1068
[19]  
Townes C.W., 1955, MICROWAVE SPECTROSCO
[20]   LABORATORY OBSERVATION OF MASER ACTION IN NH3 THROUGH COLLISIONAL COOLING [J].
WILLEY, DR ;
SOUTHWICK, RJ ;
RAMADAS, K ;
RAPELA, BK ;
NEFF, WA .
PHYSICAL REVIEW LETTERS, 1995, 74 (26) :5216-5219