共 53 条
Molecular Packing of High-Mobility Diketo Pyrrolo-Pyrrole Polymer Semiconductors with Branched Alkyl Side Chains
被引:381
作者:

Zhang, Xinran
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h-index: 0
机构:
NIST, Div Polymers, Gaithersburg, MD 20899 USA NIST, Div Polymers, Gaithersburg, MD 20899 USA

Richter, Lee J.
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h-index: 0
机构:
NIST, Surface & Microanal Sci Div, Gaithersburg, MD 20899 USA NIST, Div Polymers, Gaithersburg, MD 20899 USA

DeLongchamp, Dean M.
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h-index: 0
机构:
NIST, Div Polymers, Gaithersburg, MD 20899 USA NIST, Div Polymers, Gaithersburg, MD 20899 USA

Kline, R. Joseph
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h-index: 0
机构:
NIST, Div Polymers, Gaithersburg, MD 20899 USA NIST, Div Polymers, Gaithersburg, MD 20899 USA

Hammond, Matthew R.
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机构:
NIST, Div Polymers, Gaithersburg, MD 20899 USA NIST, Div Polymers, Gaithersburg, MD 20899 USA

McCulloch, Iain
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h-index: 0
机构:
Univ London Imperial Coll Sci Technol & Med, Dept Chem, London SW7 2AZ, England
Univ London Imperial Coll Sci Technol & Med, Ctr Plast Elect, London SW7 2AZ, England NIST, Div Polymers, Gaithersburg, MD 20899 USA

Heeney, Martin
论文数: 0 引用数: 0
h-index: 0
机构:
Univ London Imperial Coll Sci Technol & Med, Dept Chem, London SW7 2AZ, England
Univ London Imperial Coll Sci Technol & Med, Ctr Plast Elect, London SW7 2AZ, England NIST, Div Polymers, Gaithersburg, MD 20899 USA

Ashraf, Raja S.
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h-index: 0
机构:
Univ London Imperial Coll Sci Technol & Med, Dept Chem, London SW7 2AZ, England
Univ London Imperial Coll Sci Technol & Med, Ctr Plast Elect, London SW7 2AZ, England NIST, Div Polymers, Gaithersburg, MD 20899 USA

Smith, Jeremy N.
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Univ London Imperial Coll Sci Technol & Med, Ctr Plast Elect, London SW7 2AZ, England
Univ London Imperial Coll Sci Technol & Med, Dept Phys, London SW7 2AZ, England NIST, Div Polymers, Gaithersburg, MD 20899 USA

Anthopoulos, Thomas D.
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h-index: 0
机构:
Univ London Imperial Coll Sci Technol & Med, Ctr Plast Elect, London SW7 2AZ, England
Univ London Imperial Coll Sci Technol & Med, Dept Phys, London SW7 2AZ, England NIST, Div Polymers, Gaithersburg, MD 20899 USA

Schroeder, Bob
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h-index: 0
机构:
Univ Libre Bruxelles, Fac Sci, Lab Chim Polymeres, B-1050 Brussels, Belgium NIST, Div Polymers, Gaithersburg, MD 20899 USA

Geerts, Yves H.
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h-index: 0
机构:
Univ Libre Bruxelles, Fac Sci, Lab Chim Polymeres, B-1050 Brussels, Belgium NIST, Div Polymers, Gaithersburg, MD 20899 USA

Fischer, Daniel A.
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h-index: 0
机构:
NIST, Div Ceram, Gaithersburg, MD 20899 USA NIST, Div Polymers, Gaithersburg, MD 20899 USA

Toney, Michael F.
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h-index: 0
机构:
Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA 94025 USA NIST, Div Polymers, Gaithersburg, MD 20899 USA
机构:
[1] NIST, Div Polymers, Gaithersburg, MD 20899 USA
[2] NIST, Surface & Microanal Sci Div, Gaithersburg, MD 20899 USA
[3] NIST, Div Ceram, Gaithersburg, MD 20899 USA
[4] Univ London Imperial Coll Sci Technol & Med, Dept Chem, London SW7 2AZ, England
[5] Univ London Imperial Coll Sci Technol & Med, Ctr Plast Elect, London SW7 2AZ, England
[6] Univ London Imperial Coll Sci Technol & Med, Dept Phys, London SW7 2AZ, England
[7] Univ Libre Bruxelles, Fac Sci, Lab Chim Polymeres, B-1050 Brussels, Belgium
[8] Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA 94025 USA
关键词:
FIELD-EFFECT TRANSISTORS;
THIN-FILM TRANSISTORS;
HIGH-PERFORMANCE;
CHARGE-TRANSPORT;
CARRIER MOBILITY;
COPOLYMERS;
POLY(3-ALKYLTHIOPHENES);
MORPHOLOGY;
TEXTURE;
ORDER;
D O I:
10.1021/ja204515s
中图分类号:
O6 [化学];
学科分类号:
0703 ;
摘要:
We describe a series of highly soluble diketo pyrrolo-pyrrole (DPP)-bithiophene copolymers exhibiting field effect hole mobilities up to 0.74 cm(2) V(-1) s(-1), with a common synthetic motif of bulky 2-octyldodecyl side groups on the conjugated backbone. Spectroscopy, diffraction, and microscopy measurements reveal a transition in molecular packing behavior from a preferentially edge-on orientation of the conjugated plane to a preferentially face-on orientation as the attachment density of the side chains increases. Thermal annealing generally reduces both the face-on population and the misoriented edge-on domains. The highest hole mobilities of this series were obtained from edge-on molecular packing and in-plane liquid-crystalline texture, but films with a bimodal orientation distribution and no discernible in-plane texture exhibited surprisingly comparable mobilities. The high hole mobility may therefore arise from the molecular packing feature common to the entire polymer series: backbones that are strictly oriented parallel to the substrate plane and coplanar with other backbones in the same layer.
引用
收藏
页码:15073 / 15084
页数:12
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McCulloch, Iain
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机构:
Univ London Imperial Coll Sci Technol & Med, Dept Chem, London SW7 2AZ, England Natl Inst Stand & Technol, Gaithersburg, MD 20899 USA
[10]
High carrier mobility polythiophene thin films: Structure determination by experiment and theory
[J].
DeLongchamp, Dean M.
;
Kline, R. Joseph
;
Lin, Eric K.
;
Fischer, Daniel A.
;
Richter, Lee J.
;
Lucas, Leah A.
;
Heeney, Martin
;
McCulloch, Iain
;
Northrup, John E.
.
ADVANCED MATERIALS,
2007, 19 (06)
:833-+

DeLongchamp, Dean M.
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Natl Inst Stand & Technol, Gaithersburg, MD 20899 USA Natl Inst Stand & Technol, Gaithersburg, MD 20899 USA

Kline, R. Joseph
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机构: Natl Inst Stand & Technol, Gaithersburg, MD 20899 USA

Lin, Eric K.
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机构: Natl Inst Stand & Technol, Gaithersburg, MD 20899 USA

Fischer, Daniel A.
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机构: Natl Inst Stand & Technol, Gaithersburg, MD 20899 USA

Richter, Lee J.
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机构: Natl Inst Stand & Technol, Gaithersburg, MD 20899 USA

Lucas, Leah A.
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机构: Natl Inst Stand & Technol, Gaithersburg, MD 20899 USA

Heeney, Martin
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机构: Natl Inst Stand & Technol, Gaithersburg, MD 20899 USA

McCulloch, Iain
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机构: Natl Inst Stand & Technol, Gaithersburg, MD 20899 USA

Northrup, John E.
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机构: Natl Inst Stand & Technol, Gaithersburg, MD 20899 USA