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Thieno[3,2-b]thiophene-Diketopyrrolopyrrole-Containing Polymers for High-Performance Organic Field-Effect Transistors and Organic Photovoltaic Devices
被引:834
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Chen, Zhuoying
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Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England Univ London Imperial Coll Sci Technol & Med, London SW7 2AZ, England

Ashraf, Rap Shahid
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Univ London Imperial Coll Sci Technol & Med, London SW7 2AZ, England Univ London Imperial Coll Sci Technol & Med, London SW7 2AZ, England

Zhang, Weimin
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Univ London Imperial Coll Sci Technol & Med, London SW7 2AZ, England Univ London Imperial Coll Sci Technol & Med, London SW7 2AZ, England

Du, Junping
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Univ London Imperial Coll Sci Technol & Med, London SW7 2AZ, England Univ London Imperial Coll Sci Technol & Med, London SW7 2AZ, England

Durrant, James R.
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Univ London Imperial Coll Sci Technol & Med, London SW7 2AZ, England Univ London Imperial Coll Sci Technol & Med, London SW7 2AZ, England

Tuladhar, Pabitra Shakya
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Univ London Imperial Coll Sci Technol & Med, London SW7 2AZ, England Univ London Imperial Coll Sci Technol & Med, London SW7 2AZ, England

Song, Kigook
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Kyung Hee Univ, Yongin 446701, Gyeonggi Do, South Korea Univ London Imperial Coll Sci Technol & Med, London SW7 2AZ, England

Watkins, Scott E.
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机构: Univ London Imperial Coll Sci Technol & Med, London SW7 2AZ, England

Geerts, Yves
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Univ Libre Bruxelles, B-1050 Brussels, Belgium Univ London Imperial Coll Sci Technol & Med, London SW7 2AZ, England

Wienk, Martijn M.
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Eindhoven Univ Technol, NL-5600 MB Eindhoven, Netherlands Univ London Imperial Coll Sci Technol & Med, London SW7 2AZ, England

Janssen, Rene A. J.
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Eindhoven Univ Technol, NL-5600 MB Eindhoven, Netherlands Univ London Imperial Coll Sci Technol & Med, London SW7 2AZ, England

Anthopoulos, Thomas
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Univ London Imperial Coll Sci Technol & Med, London SW7 2AZ, England Univ London Imperial Coll Sci Technol & Med, London SW7 2AZ, England

Sirringhaus, Henning
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Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England Univ London Imperial Coll Sci Technol & Med, London SW7 2AZ, England

Heeney, Martin
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Univ London Imperial Coll Sci Technol & Med, London SW7 2AZ, England Univ London Imperial Coll Sci Technol & Med, London SW7 2AZ, England

McCulloch, Iain
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Univ London Imperial Coll Sci Technol & Med, London SW7 2AZ, England Univ London Imperial Coll Sci Technol & Med, London SW7 2AZ, England
机构:
[1] Univ London Imperial Coll Sci Technol & Med, London SW7 2AZ, England
[2] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England
[3] Kyung Hee Univ, Yongin 446701, Gyeonggi Do, South Korea
[4] Eindhoven Univ Technol, NL-5600 MB Eindhoven, Netherlands
[5] Univ Libre Bruxelles, B-1050 Brussels, Belgium
关键词:
THIN-FILM TRANSISTORS;
EFFICIENT SOLAR-CELLS;
SEMICONDUCTING POLYMERS;
MOBILITY;
DIKETOPYRROLOPYRROLE;
DEPENDENCE;
COPOLYMER;
D O I:
10.1021/ja110619k
中图分类号:
O6 [化学];
学科分类号:
0703 ;
摘要:
We report the synthesis and polymerization of a novel thieno[3,2-b]thiophene-diketopyrrolopyrrole-based monomer. Copolymerization with thiophene afforded a polymer with a maximum hole mobility of 1.95 cm(2) V(-1) s(-1) which is the highest mobility from a polymer-based OFET reported to date. Bulk-heterojunction solar cells comprising this polymer and PC(71)BM gave a power conversion efficiency of 5.4%.
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页码:3272 / 3275
页数:4
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