Highly Stable Semiconducting Polymers Based on Thiazolothiazole

被引：100

作者：

Osaka, Itaru ^{[1
]}

Zhang, Rui ^{[1
]}

Liu, Junying ^{[1
]}

Smilgies, Detlef-M. ^{[2
]}

Kowalewski, Tomasz ^{[1
]}

McCullough, Richard D. ^{[1
]}

机构：

[1] Carnegie Mellon Univ, Dept Chem, Pittsburgh, PA 15232 USA

[2] Cornell Univ, Cornell High Energy Synchrotron Source, Ithaca, NY 14853 USA

来源：

CHEMISTRY OF MATERIALS | 2010年 / 22卷 / 14期

基金：

美国国家科学基金会;

关键词：

FIELD-EFFECT TRANSISTORS; HIGH-MOBILITY; THIOPHENE COPOLYMERS; TEMPERATURE; CHAIN;

D O I：

10.1021/cm101052b

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

New thiazolothiazole-thiophene copolymers show high mobilities of ∼0.1 cm2/(V s) despite the fact that the polymer chains are disordered. The polymers demonstrated excellent stability, as they maintained the initial OFET performance after 50 days in ambient air (30-50% humidity). © 2010 American Chemical Society.

引用

收藏

页码：4191 / 4196

页数：6

相关论文

共 28 条

[1] High-performance plastic transistors fabricated by printing techniques [J].

Bao, ZN ;

Feng, Y ;

Dodabalapur, A ;

Raju, VR ;

Lovinger, AJ .

CHEMISTRY OF MATERIALS, 1997, 9 (06) :1299-&

[2] X-ray scattering study of thin films of poly(2,5-bis(3-alkylthiophen-2-yl)thieno[3,2-b]thiophene) [J].

Chabinyc, Michael L. ;

Toney, Michael F. ;

Kline, R. Joseph ;

McCulloch, Iain ;

Heeney, Martin .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2007, 129 (11) :3226-3237

[3] Effects of humidity on unencapsulated poly(thiophene) thin-film transistors [J].

Chabinyc, ML ;

Endicott, F ;

Vogt, BD ;

DeLongchamp, DM ;

Lin, EK ;

Wu, YL ;

Liu, P ;

Ong, BS .

APPLIED PHYSICS LETTERS, 2006, 88 (11)

[4] Large-scale complementary integrated circuits based on organic transistors [J].

Crone, B ;

Dodabalapur, A ;

Lin, YY ;

Filas, RW ;

Bao, Z ;

LaDuca, A ;

Sarpeshkar, R ;

Katz, HE ;

Li, W .

NATURE, 2000, 403 (6769) :521-523

[5] Tetrathienoacene copolymers as high mobility, soluble organic semiconductors [J].

Fong, Hon Hang ;

Pozdin, Vladimir A. ;

Amassian, Aram ;

Malliaras, George G. ;

Smilgies, Detlef-M. ;

He, Mingqian ;

Gasper, Susan ;

Zhang, Feixia ;

Sorensen, Michael .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2008, 130 (40) :13202-13203

[6] ALL-POLYMER FIELD-EFFECT TRANSISTOR REALIZED BY PRINTING TECHNIQUES [J].

GARNIER, F ;

HAJLAOUI, R ;

YASSAR, A ;

SRIVASTAVA, P .

SCIENCE, 1994, 265 (5179) :1684-1686

[7] Chiral polymerization - Optically active conjugated polymers prepared from achiral monomers by polycondensation in a chiral nematic solvent [J].

Goto, H ;

Akagi, K .

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2005, 44 (28) :4322-4328

[8] Stable polythiophene semiconductors incorporating thieno[2,3-b]thiophene [J].

Heeney, M ;

Bailey, C ;

Genevicius, K ;

Shkunov, M ;

Sparrowe, D ;

Tierney, S ;

McCulloch, I .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2005, 127 (04) :1078-1079

[9]

Klauk H., 2006, Organic Electronics

[10] Field-effect transistors based on thiophene hexamer analogues with diminished electron donor strength [J].

Li, WJ ;

Katz, HE ;

Lovinger, AJ ;

Laquindanum, JG .

CHEMISTRY OF MATERIALS, 1999, 11 (02) :458-465