Pyro-cumulonimbus injection of smoke to the stratosphere: Observations and impact of a super blowup in northwestern Canada on 3-4 August 1998

被引:141
作者
Fromm, M
Bevilacqua, R
Servranckx, R
Rosen, J
Thayer, JP
Herman, J
Larko, D
机构
[1] USN, Res Lab, Washington, DC 20375 USA
[2] Canadian Meteorol Ctr, Dorval, PQ H9P 1J3, Canada
[3] Univ Wyoming, Dept Phys & Astron, Dept 3905, Laramie, WY 82071 USA
[4] Univ Colorado, Dept Aerosp Engn Sci, Ctr Engn, Boulder, CO 80309 USA
[5] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA
[6] Sci Syst & Applicat Inc, Lanham, MD 20706 USA
关键词
D O I
10.1029/2004JD005350
中图分类号
P4 [大气科学(气象学)];
学科分类号
0706 ; 070601 ;
摘要
We report observations and analysis of a pyro-cumulonimbus event in the midst of a boreal forest fire blowup in Northwest Territories Canada, near Norman Wells, on 3-4 August 1998. We find that this blowup caused a five-fold increase in lower stratospheric aerosol burden, as well as multiple reports of anomalous enhancements of tropospheric gases and aerosols across Europe 1 week later. Our observations come from solar occultation satellites (POAM III and SAGE II), nadir imagers (GOES, AVHRR, SeaWiFS, DMSP), TOMS, lidar, and backscattersonde. First, we provide a detailed analysis of the 3 August eruption of extreme pyro-convection. This includes identifying the specific pyro-cumulonimbus cells that caused the lower stratospheric aerosol injection, and a meteorological analysis. Next, we characterize the altitude, composition, and opacity of the post-convection smoke plume on 4-7 August. Finally, the stratospheric impact of this injection is analyzed. Satellite images reveal two noteworthy pyro-cumulonimbus phenomena: (1) an active-convection cloud top containing enough smoke to visibly alter the reflectivity of the cloud anvil in the Upper Troposphere Lower Stratosphere (UTLS) and (2) a smoke plume, that endured for at least 2 hours, atop an anvil. The smoke pall deposited by the Norman Wells pyro-convection was a very large, optically dense, UTLS-level plume on 4 August that exhibited a mesoscale cyclonic circulation. An analysis of plume color/texture from SeaWiFS data, aerosol index, and brightness temperature establishes the extreme altitude and "pure" smoke composition of this unique plume. We show what we believe to be a first-ever measurement of strongly enhanced ozone in the lower stratosphere mingled with smoke layers. We conclude that two to four extreme pyro-thunderstorms near Norman Wells created a smoke injection of hemispheric scope that substantially increased stratospheric optical depth, transported aerosols 7 km above the tropopause (above similar to 430 K potential temperature), and also perturbed lower stratospheric ozone.
引用
收藏
页码:1 / 17
页数:16
相关论文
共 39 条
[11]   An analysis of Polar Ozone and Aerosol Measurement (POAM) II Arctic polar stratospheric cloud observations, 1993-1996 [J].
Fromm, MD ;
Bevilacqua, RM ;
Hornstein, J ;
Shettle, E ;
Hoppel, K ;
Lumpe, JD .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1999, 104 (D20) :24341-24357
[12]   STRATOSPHERE-TROPOSPHERE EXCHANGE [J].
HOLTON, JR ;
HAYNES, PH ;
MCINTYRE, ME ;
DOUGLASS, AR ;
ROOD, RB ;
PFISTER, L .
REVIEWS OF GEOPHYSICS, 1995, 33 (04) :403-439
[13]   Comparisons of the TOMS aerosol index with Sun-photometer aerosol optical thickness: Results and applications [J].
Hsu, NC ;
Herman, JR ;
Torres, O ;
Holben, BN ;
Tanre, D ;
Eck, TF ;
Smirnov, A ;
Chatenet, B ;
Lavenu, F .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1999, 104 (D6) :6269-6279
[14]   Satellite detection of smoke aerosols over a snow/ice surface by TOMS [J].
Hsu, NC ;
Herman, JR ;
Gleason, JF ;
Torres, O ;
Seftor, CJ .
GEOPHYSICAL RESEARCH LETTERS, 1999, 26 (08) :1165-1168
[15]   In-situ observations of mid-latitude forest fire plumes deep in the stratosphere [J].
Jost, HJ ;
Drdla, K ;
Stohl, A ;
Pfister, L ;
Loewenstein, M ;
Lopez, JP ;
Hudson, PK ;
Murphy, DM ;
Cziczo, DJ ;
Fromm, M ;
Bui, TP ;
Dean-Day, J ;
Gerbig, C ;
Mahoney, MJ ;
Richard, EC ;
Spichtinger, N ;
Pittman, JV ;
Weinstock, EM ;
Wilson, JC ;
Xueref, I .
GEOPHYSICAL RESEARCH LETTERS, 2004, 31 (11) :L111011-5
[16]   Improving global estimates of atmospheric emissions from biomass burning [J].
Kasischke, ES ;
Penner, JE .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2004, 109 (D14) :D14S01
[17]  
KASISCHKE ES, 1999, EOS, V80, P143
[18]   International Geosphere-Biosphere Programme International Global Atmospheric Chemistry SAFARI-92 field experiment: Background and overview [J].
Lindesay, JA ;
Andreae, MO ;
Goldammer, JG ;
Harris, G ;
Annegarn, HJ ;
Garstang, M ;
Scholes, RJ ;
vanWilgen, BW .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1996, 101 (D19) :23521-23530
[19]   Enhancements in lower stratospheric CH3CN observed by the upper atmosphere research satellite microwave limb sounder following boreal forest fires -: art. no. D06308 [J].
Livesey, NJ ;
Fromm, MD ;
Waters, JW ;
Manney, GL ;
Santee, ML ;
Read, WG .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2004, 109 (D6)
[20]   The Polar Ozone and Aerosol Measurement (POAM) III instrument and early validation results [J].
Lucke, RL ;
Korwan, DR ;
Bevilacqua, RM ;
Hornstein, JS ;
Shettle, EP ;
Chen, DT ;
Daehler, M ;
Lumpe, JD ;
Fromm, MD ;
Debrestian, D ;
Neff, B ;
Squire, M ;
König-Langlo, G ;
Davies, J .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1999, 104 (D15) :18785-18799