Catalytic Action of a Cu(111) Surface on Tetraazaperopyrene Polymerization

被引：14

作者：

Blankenburg, S. ^{[1
]}

Rauls, E. ^{[1
]}

Schmidt, W. G. ^{[1
]}

机构：

[1] Univ Paderborn, Lehrstuhl Theoret Phys, D-33095 Paderborn, Germany

来源：

JOURNAL OF PHYSICAL CHEMISTRY LETTERS | 2010年 / 1卷 / 22期

关键词：

FABRICATION; MOLECULES; GRAPHENE;

D O I：

10.1021/jz101389u

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

The polymerization of tetraazaperopyrene molecules on a Cu(111) substrate, as observed in recent scanning tunneling microscopy experiments, has been investigated in detail by first-priniciples calculation. Tautomerization is the first step required for the formation of molecular dimers and polymers. The substrate has been found to catalyze this tautomerization.

引用

页码：3266 / 3270

页数：5

共 26 条

[1]

[Anonymous], 2009, Angew. Chem

[2] Molecular architectonic on metal surfaces [J].

Barth, Johannes V. .

ANNUAL REVIEW OF PHYSICAL CHEMISTRY, 2007, 58 :375-407

[3] Porous graphenes: two-dimensional polymer synthesis with atomic precision [J].

Bieri, Marco ;

Treier, Matthias ;

Cai, Jinming ;

Ait-Mansour, Kamel ;

Ruffieux, Pascal ;

Groening, Oliver ;

Groening, Pierangelo ;

Kastler, Marcel ;

Rieger, Ralph ;

Feng, Xinliang ;

Muellen, Klaus ;

Fasel, Roman .

CHEMICAL COMMUNICATIONS, 2009, (45) :6919-6921

[4] STM fingerprint of molecule-adatom interactions in a self-assembled metal-organic surface coordination network on Cu(111) [J].

Bjork, Jonas ;

Matena, Manfred ;

Dyer, Matthew S. ;

Enache, Mihaela ;

Lobo-Checa, Jorge ;

Gade, Lutz H. ;

Jung, Thomas A. ;

Stohr, Meike ;

Persson, Mats .

PHYSICAL CHEMISTRY CHEMICAL PHYSICS, 2010, 12 (31) :8815-8821

[5] Long-range chiral recognition due to substrate locking and substrate-adsorbate charge transfer [J].

Blankenburg, S. ;

Schmidt, W. G. .

PHYSICAL REVIEW LETTERS, 2007, 99 (19)

[6] Steric effects and chirality in the adsorption of glycine and phenylglycine on Cu(110) [J].

Blankenburg, S. ;

Schmidt, W. G. .

NANOTECHNOLOGY, 2007, 18 (42)

[7] Role of Dihydrogen Bonds for the Stabilization of Self-Assembled Molecular Nanostructures [J].

Blankenburg, S. ;

Rauls, E. ;

Schmidt, W. G. .

JOURNAL OF PHYSICAL CHEMISTRY C, 2009, 113 (29) :12653-12657

[8] Spatial modulation of molecular adsorption energies due to indirect interaction [J].

Blankenburg, S. ;

Schmidt, W. G. .

PHYSICAL REVIEW B, 2008, 78 (23)

[9] Porous Graphene as an Atmospheric Nanofilter [J].

Blankenburg, Stephan ;

Bieri, Marco ;

Fasel, Roman ;

Muellen, Klaus ;

Pignedoli, Carlo A. ;

Passerone, Daniele .

SMALL, 2010, 6 (20) :2266-2271

[10] Atomically precise bottom-up fabrication of graphene nanoribbons [J].

Cai, Jinming ;

Ruffieux, Pascal ;

Jaafar, Rached ;

Bieri, Marco ;

Braun, Thomas ;

Blankenburg, Stephan ;

Muoth, Matthias ;

Seitsonen, Ari P. ;

Saleh, Moussa ;

Feng, Xinliang ;

Muellen, Klaus ;

Fasel, Roman .

NATURE, 2010, 466 (7305) :470-473

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