Characterization of an atmospheric pressure dc plasma jet

被引:36
作者
Bibinov, N. [1 ]
Dudek, D. [2 ]
Awakowicz, P. [1 ]
Engemann, J. [2 ]
机构
[1] Ruhr Univ Bochum, Inst Elect Engn & Plasma, D-44780 Bochum, Germany
[2] Wuppertal Univ, Microstruct Res Ctr, D-42119 Wuppertal, Germany
关键词
D O I
10.1088/0022-3727/40/23/018
中图分类号
O59 [应用物理学];
学科分类号
摘要
The fluxes of chemical active particles in the effluent of plasma jets are very important parameters for different applications. Herein, we present a method of measurement and an algorithm to obtain plasma parameters and particle fluxes from the atmospheric pressure direct current (dc) plasma jet operated in nitrogen/oxygen mixtures. We determine the atom and radical steady state densities and particles fluxes by means of emission spectroscopy and numerical modelling. The plasma parameters, electron density ne and electron velocity distribution function, are obtained by means of emission spectroscopy, microphotography and solutions of the Boltzmann equation. The steady state densities of particles in the effluent region are calculated by solving transport equations (thermal conductivity and diffusion) and chemical kinetics equations. The calculated densities of nitrogen atoms are compared with emission spectroscopy measurements at various positions outside the nozzle of the plasma source. The measurements confirm model results. The fluxes of chemically active particles are determined by means of steady state particle densities and known gas flow rate.
引用
收藏
页码:7372 / 7378
页数:7
相关论文
共 24 条
[1]   EVALUATED KINETIC AND PHOTOCHEMICAL DATA FOR ATMOSPHERIC CHEMISTRY .3. IUPAC SUBCOMMITTEE ON GAS KINETIC DATA EVALUATION FOR ATMOSPHERIC CHEMISTRY [J].
ATKINSON, R ;
BAULCH, DL ;
COX, RA ;
HAMPSON, RF ;
KERR, JA ;
TROE, J .
JOURNAL OF PHYSICAL AND CHEMICAL REFERENCE DATA, 1989, 18 (02) :881-1097
[2]   Relative and absolute intensity calibrations of a modern broadband echelle spectrometer [J].
Bibinov, N. ;
Halfmann, H. ;
Awakowicz, P. ;
Wiesemann, K. .
MEASUREMENT SCIENCE AND TECHNOLOGY, 2007, 18 (05) :1327-1337
[3]   A simulation study of the digital ion trap mass spectrometer [J].
Ding, L ;
Sudakov, M ;
Kumashiro, S .
INTERNATIONAL JOURNAL OF MASS SPECTROMETRY, 2002, 221 (02) :117-138
[4]   Direct current plasma jet needle source [J].
Dudek, D. ;
Bibinov, N. ;
Engemann, J. ;
Awakowicz, P. .
JOURNAL OF PHYSICS D-APPLIED PHYSICS, 2007, 40 (23) :7367-7371
[5]   PRODUCT BRANCHING RATIOS FROM THE N-2(A3-SIGMA-U+)+O-2 INTERACTION [J].
FRASER, ME ;
PIPER, LG .
JOURNAL OF PHYSICAL CHEMISTRY, 1989, 93 (03) :1107-1111
[6]   Self-consistent electron and heavy-particle kinetics in a low-pressure N-2-O-2 glow discharge [J].
Guerra, V ;
Loureiro, J .
PLASMA SOURCES SCIENCE & TECHNOLOGY, 1997, 6 (03) :373-385
[7]   Evaluated chemical kinetics data for reactions of N(2D), N(2P), and N2(A3Σu+) in the gas phase [J].
Herron, JT .
JOURNAL OF PHYSICAL AND CHEMICAL REFERENCE DATA, 1999, 28 (05) :1453-1483
[8]   CROSS-SECTIONS FOR COLLISIONS OF ELECTRONS AND PHOTONS WITH OXYGEN MOLECULES [J].
ITIKAWA, Y ;
ICHIMURA, A ;
ONDA, K ;
SAKIMOTO, K ;
TAKAYANAGI, K ;
HATANO, Y ;
HAYASHI, M ;
NISHIMURA, H ;
TSURUBUCHI, S .
JOURNAL OF PHYSICAL AND CHEMICAL REFERENCE DATA, 1989, 18 (01) :23-42
[9]   Cross sections for electron collisions with nitrogen molecules [J].
Itikawa, Y .
JOURNAL OF PHYSICAL AND CHEMICAL REFERENCE DATA, 2006, 35 (01) :31-53
[10]  
KOHLRAUSCH F, 1996, PRAKTISCHE PHYS, V3, P356