H2O splitting in tubular plasma reactors

被引：32

作者：

Chen, X

Marquez, M

Rozak, J

Marun, C

Luo, J

Suib, SL

Hayashi, Y

Matsumoto, H

机构：

[1] Univ Connecticut, Dept Chem, Storrs, CT 06269 USA

[2] Univ Connecticut, Dept Chem Engn, Storrs, CT 06269 USA

[3] Univ Connecticut, Inst Mat Sci, Storrs, CT 06269 USA

[4] Yale Univ, Dept Appl Phys & Elect Engn, New Haven, CT 06511 USA

来源：

JOURNAL OF CATALYSIS | 1998年 / 178卷 / 01期

关键词：

D O I：

10.1006/jcat.1998.2120

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

Significant hydrogen productivity (0.33 mol% in products) from H2O splitting by atmospheric dielectric barrier discharges has been achieved with tubular plasma reactors at room temperature. The water splitting activity varies with different metal-coated inner electrodes and different peak voltages across the reactor. An optimal emission spectroscopic study was performed in order to explain the metal effect. O*/Ar* emission intensity ratio as well as excitation temperatures were used for rationalizing the metal effect. (C) 1998 Academic Press.

引用

页码：372 / 377

页数：6

共 14 条

[1]

AMOUYAL E, 1995, SOL ENERG MAT SOL C, V94, P8028

[2] Catalysis and plasma chemistry at solid surfaces [J].