Fluorescence imaging and time-resolved fluorescence measurement of dye molecules with a flexible molecular structure were carried out at a single-molecule level on a poly(methyl methacrylate) film. The nonexponential fluorescence decay curves observed in the conventional bulk measurements were attributed to the site-dependent nonradiative process of the individual dye molecules. Owing to the site-sensitive nature of the crystal violet molecules used, a bimodal site distribution of the polymer film was revealed based on the single-molecule measurements. (C) 1998 Elsevier Science B.V. All rights reserved.
机构:
UNIV CALIF BERKELEY LAWRENCE BERKELEY LAB, DIV MAT & MOLEC RES, BERKELEY, CA 94720 USAUNIV CALIF BERKELEY LAWRENCE BERKELEY LAB, DIV MAT & MOLEC RES, BERKELEY, CA 94720 USA
BENAMOTZ, D
HARRIS, CB
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UNIV CALIF BERKELEY LAWRENCE BERKELEY LAB, DIV MAT & MOLEC RES, BERKELEY, CA 94720 USAUNIV CALIF BERKELEY LAWRENCE BERKELEY LAB, DIV MAT & MOLEC RES, BERKELEY, CA 94720 USA
机构:
UNIV CALIF BERKELEY LAWRENCE BERKELEY LAB, DIV MAT & MOLEC RES, BERKELEY, CA 94720 USAUNIV CALIF BERKELEY LAWRENCE BERKELEY LAB, DIV MAT & MOLEC RES, BERKELEY, CA 94720 USA
BENAMOTZ, D
HARRIS, CB
论文数: 0引用数: 0
h-index: 0
机构:
UNIV CALIF BERKELEY LAWRENCE BERKELEY LAB, DIV MAT & MOLEC RES, BERKELEY, CA 94720 USAUNIV CALIF BERKELEY LAWRENCE BERKELEY LAB, DIV MAT & MOLEC RES, BERKELEY, CA 94720 USA