Controlling the interactions between polaritons and molecular vibrations in strongly coupled organic semiconductor microcavities

被引：35

作者：

Chovan, J. ^{[1
,2
]}

Perakis, I. E. ^{[1
,2
]}

Ceccarelli, S. ^{[3
]}

Lidzey, D. G. ^{[3
]}

机构：

[1] Univ Crete, Inst Elect Struct & Laser, Fdn Res & Technol Hellas, Iraklion 71003, Crete, Greece

[2] Univ Crete, Dept Phys, Iraklion 71003, Crete, Greece

[3] Univ Sheffield, Dept Phys & Astron, Sheffield S3 7RH, S Yorkshire, England

来源：

PHYSICAL REVIEW B | 2008年 / 78卷 / 04期

关键词：

D O I：

10.1103/PhysRevB.78.045320

中图分类号：

T [工业技术];

学科分类号：

08 ;

摘要：

We study the microscopic processes that determine the dynamics of polaritons in strongly-coupled organic-semiconductor microcavities. Using a quantum kinetic theory, we show that resonant couplings and interactions between cavity photons, excitons, and localized molecular vibrations strongly affect the polariton resonance line shapes in J-aggregate microcavities. We use our many-body calculation to reproduce the measured polariton emission at exciton-photon resonance which is determined as a function of the Rabi-splitting energy.

引用

页数：5

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