Promises and challenges of perovskite solar cells

被引：1756

作者：

Correa-Baena, Juan-Pablo ^{[1
,2
]}

Saliba, Michael ^{[2
]}

Buonassisi, Tonio ^{[1
]}

Graetzel, Michael ^{[2
]}

Abate, Antonio ^{[3
]}

Tress, Wolfgang ^{[2
]}

Hagfeldt, Anders ^{[2
]}

机构：

[1] MIT, 77 Massachusetts Ave, Cambridge, MA 02139 USA

[2] Ecole Polytech Fed Lausanne, CH-1015 Lausanne, Switzerland

[3] Helmholtz Zentrum Berlin Mat & Energie, D-12489 Berlin, Germany

来源：

SCIENCE | 2017年 / 358卷 / 6364期

关键词：

HALIDE PEROVSKITES; EFFICIENT; PERFORMANCE; TRANSPORT; PHOTOVOLTAICS; FORMAMIDINIUM; MIGRATION; ELECTRON; IODIDE; LAYERS;

D O I：

10.1126/science.aam6323

中图分类号：

O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];

学科分类号：

07 ; 0710 ; 09 ;

摘要：

The efficiencies of perovskite solar cells have gone from single digits to a certified 22.1% in a few years' time. At this stage of their development, the key issues concern how to achieve further improvements in efficiency and long-term stability. We review recent developments in the quest to improve the current state of the art. Because photocurrents are near the theoretical maximum, our focus is on efforts to increase open-circuit voltage by means of improving charge-selective contacts and charge carrier lifetimes in perovskites via processes such as ion tailoring. The challenges associated with long-term perovskite solar cell device stability include the role of testing protocols, ionic movement affecting performance metrics over extended periods of time, and determination of the best ways to counteract degradation mechanisms.

引用

页码：739 / 744

页数：6

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