Indoor and outdoor carbonyl compounds in the hotel ballrooms in Guangzhou, China

被引:94
作者
Feng, YL [1 ]
Wen, S [1 ]
Wang, XM [1 ]
Sheng, GY [1 ]
He, QS [1 ]
Tang, JH [1 ]
Fu, JM [1 ]
机构
[1] Chinese Acad Sci, Guangzhou Inst Geochem, Guagzhou Key Lab Environm Protect & Resources Uti, State Key Lab Organ Geochem, Guangzhou 510640, Peoples R China
关键词
carbonyls; photochemical reactions; high molecular weight (HMW); sources; exposure;
D O I
10.1016/j.atmosenv.2003.09.061
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Twenty-one carbonyl compounds were measured simultaneously at four hotel ballrooms in urban Guangzhou during the autumn, 2002. In each ballroom, measurements were carried out in business hours in the evening (20:30-24:00) on 7 consecutive days without any disturbance of the ballroom's normal operation. Nineteen out of the 21 target carbonyl compounds were identified in indoor and outdoor air. In the outdoor environment, formaldehyde was the most abundant carbonyl, followed by acetaldehyde, and there existed a strong correlation between formaldehyde and acetaldehyde. In the indoor air, however, acetaldehyde was the most abundant carbonyl, its concentrations seemed to be affected significantly by smoking. The indoor concentrations of carbonyls were found higher than their outdoor counterparts with only a few exceptions. Further studies concerning the indoor/outdoor ratios and mutual correlation of the carbonyls indicated that apart from direct emission from indoor materials and infiltration of outdoor air, other anthropogenic sources, e.g. tobacco smoke, also significantly contributed to carbonyl compounds. The possible sources of some high molecular weight carbonyls, e.g. nonanaldehyde, were also discussed briefly. Preliminary estimate of the exposures and risks due to carbonyls in the ballrooms was made, which indicated that long-term exposure in such places might cause increased chance of developing cancers. (C) 2003 Elsevier Ltd. All rights reserved.
引用
收藏
页码:103 / 112
页数:10
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