Ordering in stretch-tunable polymeric opal fibers

被引:76
作者
Finlayson, Chris E. [1 ]
Goddard, Chris [2 ]
Papachristodoulou, Elpida [1 ]
Snoswell, David R. E. [1 ]
Kontogeorgos, Andreas [1 ]
Spahn, Peter [3 ]
Hellmann, G. P. [3 ]
Hess, Ortwin [2 ]
Baumberg, Jeremy J. [1 ]
机构
[1] Univ Cambridge, NanoPhoton Ctr, Cambridge CB3 0HE, England
[2] Univ London Imperial Coll Sci Technol & Med, Blackett Lab, London SW7 2AZ, England
[3] DKI, D-64289 Darmstadt, Germany
来源
OPTICS EXPRESS | 2011年 / 19卷 / 04期
基金
英国工程与自然科学研究理事会;
关键词
SHEAR-INDUCED ORDER; COMPUTER EXPERIMENTS; COLLOIDAL CRYSTALS; PHOTONIC CRYSTALS; CLASSICAL FLUIDS; SUSPENSIONS;
D O I
10.1364/OE.19.003144
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
We demonstrate the production of high-quality polymer opal fibers in an industrially-scalable process. These fibers exhibit structural color, based on the self-assembly of sub-micron core-shell particles, with a spectrum which is stretch-tunable across the visible region. The internal substructure and ordering of fibers, as inferred from variations in spectral bandwidth, is studied using dark-field microscopy. We employ a granular model to examine flow and shear forces during the extrusion process, and the effects on particle ordering. In both theory and experiment, a concentric zone of the fiber near the exposed surface develops particularly strong structural color. Such elastically-tuned structurally colored fibers are of interest for many applications. (C)2011 Optical Society of America
引用
收藏
页码:3144 / 3154
页数:11
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