Long-range molecular resonances in a cold Rydberg gas -: art. no. 183002

被引:103
作者
Farooqi, SM [1 ]
Tong, D [1 ]
Krishnan, S [1 ]
Stanojevic, J [1 ]
Zhang, YP [1 ]
Ensher, JR [1 ]
Estrin, AS [1 ]
Boisseau, C [1 ]
Côté, R [1 ]
Eyler, EE [1 ]
Gould, PL [1 ]
机构
[1] Univ Connecticut, Dept Phys, Storrs, CT 06269 USA
关键词
D O I
10.1103/PhysRevLett.91.183002
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We present evidence for molecular resonances in a cold dense gas of rubidium Rydberg atoms. Single UV photon excitation from the 5s ground state to np Rydberg states (n=50-90) reveals resonances at energies corresponding to excited atom pairs (n-1)d+ns. We attribute these normally forbidden transitions to avoided crossings between the long-range molecular potentials of two Rydberg atoms. These strong van der Waals interactions result in avoided crossings at extremely long range, e.g., similar to58 000 times the Bohr radius (a(0)) for n=70.
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页数:4
相关论文
共 24 条
[1]   Resonant dipole-dipole energy transfer in a nearly frozen Rydberg gas [J].
Anderson, WR ;
Veale, JR ;
Gallagher, TF .
PHYSICAL REVIEW LETTERS, 1998, 80 (02) :249-252
[2]   Macrodimers:: Ultralong range Rydberg molecules -: art. no. 133004 [J].
Boisseau, C ;
Simbotin, I ;
Côté, R .
PHYSICAL REVIEW LETTERS, 2002, 88 (13) :4-133004
[3]   Energies and dipole moments of long-range molecular Rydberg states [J].
Chibisov, MI ;
Khuskivadze, AA ;
Fabrikant, II .
JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS, 2002, 35 (10) :L193-L198
[4]  
Dalgarno A., 1966, ADV ATOM MOL PHYS, V2, P1
[5]   Rydberg cold collisions dominated by ultralong range potential [J].
de Oliveira, AL ;
Mancini, MW ;
Bagnato, VS ;
Marcassa, LG .
PHYSICAL REVIEW LETTERS, 2003, 90 (14) :4
[6]   High-angular-momentum states in cold Rydberg gases [J].
Dutta, SK ;
Feldbaum, D ;
Walz-Flannigan, A ;
Guest, JR ;
Raithel, G .
PHYSICAL REVIEW LETTERS, 2001, 86 (18) :3993-3996
[7]  
Gallagher T., 1994, RYDBERG ATOMS, DOI DOI 10.1017/CBO9780511524530.021
[8]   Quantum and semiclassical analysis of long-range Rydberg molecules [J].
Granger, BE ;
Hamilton, EL ;
Greene, CH .
PHYSICAL REVIEW A, 2001, 64 (04) :425081-425089
[9]  
Greene C. H., COMMUNICATION
[10]   Creation of polar and nonpolar ultra-long-range Rydberg molecules [J].
Greene, CH ;
Dickinson, AS ;
Sadeghpour, HR .
PHYSICAL REVIEW LETTERS, 2000, 85 (12) :2458-2461